Spatial Distribution of Old and Emerging Flame Retardants in Chinese Forest Soils: Sources, Trends and Processes.
Zheng, Qian1; Nizzetto, Luca2,3; Li, Jun1; Mulder, Marie D.2; Sanka, Ondrej2; Lammel, Gerhard2,4; Bing, Haijian5; Liu, Xin1; Jiang, Yishan1; Luo, Chunling1
刊名ENVIRONMENTAL SCIENCE & TECHNOLOGY
2015-03-03
卷号49期号:5页码:2904-2911
关键词Spatial Distribution
ISSN号0013-936X
通讯作者Nizzetto, Luca
英文摘要The levels and distribution of polybrominated diphenylethers (PBDEs), novel brominated flame retardants (NBFRs) and Dechlorane Plus (DP) in soils and their dependence on environmental and anthropological factors were investigated in 159 soil samples from 30 background forested mountain sites across China. Decabromodiphenylethane (DBDPE) was the most abundant flame retardant (25-18 000 pg g(-1) and 5-13 000 pg g(-1) in O-horizon and A-horizon, respectively), followed by BDE 209 (nd-5900 pg g(-1) and nd-2400 pg g(-1) in O-horizon and A-horizon, respectively). FRs distributions were primarily controlled by source distribution. The distributions of most phasing-out PBDEs, DP isomers and TBPH were in fact correlated to a population density-based index used as proxy of areas with elevated usage and waste of FR containing products. High concentrations of some NBFRs were however observed in industrialized regions and FR manufacturing plants. Strongly positive correlations were observed between PBDEs and their replacement products suggesting similar emission pattern and environmental behavior. Exposure of mineral subsoils depended on precipitations driving leaching of FRs into the soil core. This was especially evident for some emerging BFRs (TBE, TBPH, and TBB etc.) possibly indicating potential for diffuse groundwater contamination.
WOS标题词Science & Technology ; Technology ; Life Sciences & Biomedicine
类目[WOS]Engineering, Environmental ; Environmental Sciences
研究领域[WOS]Engineering ; Environmental Sciences & Ecology
关键词[WOS]POLYBROMINATED DIPHENYL ETHERS ; PEARL RIVER DELTA ; GREAT-LAKES ATMOSPHERE ; DECHLORANE PLUS ; SOUTH CHINA ; E-WASTE ; ORGANOCHLORINE COMPOUNDS ; TIBETAN PLATEAU ; SURFACE SOILS ; UNITED-STATES
收录类别SCI
原文出处http://pubs.acs.org/doi/abs/10.1021/es505876k
语种英语
WOS记录号WOS:000350611100042
内容类型期刊论文
源URL[http://ir.imde.ac.cn/handle/131551/9593]  
专题成都山地灾害与环境研究所_山地灾害与地表过程重点实验室
成都山地灾害与环境研究所_山地表生过程与生态调控重点实验室
作者单位1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
2.Masaryk Univ, Res Ctr Tox Cpds Environm, CS-60177 Brno, Czech Republic
3.Norwegian Inst Water Res, NO-0349 Oslo, Norway
4.Max Planck Inst Chem, D-55128 Mainz, Germany
5.Chinese Acad Sci, Inst Mt Hazards & Environm, Key Lab Mt Surface Proc & Ecol Regulat, Chengdu 610041, Peoples R China
推荐引用方式
GB/T 7714
Zheng, Qian,Nizzetto, Luca,Li, Jun,et al. Spatial Distribution of Old and Emerging Flame Retardants in Chinese Forest Soils: Sources, Trends and Processes.[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2015,49(5):2904-2911.
APA Zheng, Qian.,Nizzetto, Luca.,Li, Jun.,Mulder, Marie D..,Sanka, Ondrej.,...&Zhang, Gan.(2015).Spatial Distribution of Old and Emerging Flame Retardants in Chinese Forest Soils: Sources, Trends and Processes..ENVIRONMENTAL SCIENCE & TECHNOLOGY,49(5),2904-2911.
MLA Zheng, Qian,et al."Spatial Distribution of Old and Emerging Flame Retardants in Chinese Forest Soils: Sources, Trends and Processes.".ENVIRONMENTAL SCIENCE & TECHNOLOGY 49.5(2015):2904-2911.
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