A 200-Year Record of Polycyclic Aromatic Hydrocarbons Contamination in an Ombrotrophic Peatland in Great Hinggan Mountain, Northeast China

CORC > 成都山地灾害与环境研究所 > 中国科学院水利部成都山地灾害与环境研究所 > Journal of Mountain Science > Journal of Mountain Science-2014 > Vol11 No.5

	A 200-Year Record of Polycyclic Aromatic Hydrocarbons Contamination in an Ombrotrophic Peatland in Great Hinggan Mountain, Northeast China
	BAO Kun-shan ; SHEN Ji ; ZHANG Yan ; WANG Jian ; WANG Guo-ping
刊名	Journal of Mountain Science
	2014-09
卷号	11 期号:5 页码:1085-1096
关键词	Ombrotrophic peatland polycyclic aromatic hydrocarbons (PAHs) Lead-210 Environmental pollution
通讯作者	WANG Guo-ping
英文摘要	Peat bogs are regarded as one of the faithful archives of atmospheric polycyclic aromatic hydrocarbons (PAHs) deposition, and a large number of studies on PAHs accumulation in peatlands have been reported in Europe and North America. Comparatively little information is available on peat chronological records of atmospheric PAHs flux in China. We investigated the concentrations and historical accumulation rates of PAHs (AR PAHs) through geochemical analysis of three 210Pb-dated ombrotrophic peat cores from Great Hinggan Mountain, northeast China. Eight USEPA priority PAHs were detected and they are naphthalene (Nap), acenaphthylene (Acl), acenaphthene (Ace), fluorence (Flu), phenanthrene (Phe), anthracene (Ant), fluoranthene (Fla) and pyrene (Pyr), respectively. The average total eight PAHs (tPAHs) concentrations are 135.98 - 262.43 μg kg-1 and the average AR tPAHs over the last two centuries are 96.45 - 135.98 μg m-2 yr-1. The Ace, Acl and Phe account for 30.93 - 54.04%, 25.29 - 35.81%, and 9.14 - 19.84% of the tPAHs, respectively, and have significant positive correlations with the tPAH. As a result, they are regarded as the iconic compounds of PAHs pollution in this area. A ca. 200-yr atmospheric PAHs contamination history was reconstructed from the temporal sequences of both concentration and AR tPAHs, suggesting the variation of local environmental pollution. The main sources of the PAHs are identified by two isomer ratios as petrogenic origin including oil extraction and refining process as well as their combustions for industrial development. In addition, the contribution of coal combustion for industrial activities and resident heating could not be ignored. But prior to 1860, the undeveloped industry and most of agricultural activities might mainly account for the low level of PAHs, although it could infer a long-range input of atmospheric PAHs from other industrial areas. Therefore, there is a global implication to study long-term PAHs pollution records and all the results will provide practical significance in formulating policies to achieve sustainable and healthy development.
收录类别	SCI
公开日期	2014-09-17
内容类型	期刊论文
源URL	[http://ir.imde.ac.cn/handle/131551/7240]
专题	成都山地灾害与环境研究所_Journal of Mountain Science _Journal of Mountain Science-2014_Vol11 No.5
推荐引用方式 GB/T 7714	BAO Kun-shan,SHEN Ji,ZHANG Yan,et al. A 200-Year Record of Polycyclic Aromatic Hydrocarbons Contamination in an Ombrotrophic Peatland in Great Hinggan Mountain, Northeast China[J]. Journal of Mountain Science,2014,11(5):1085-1096.
APA	BAO Kun-shan,SHEN Ji,ZHANG Yan,WANG Jian,&WANG Guo-ping.(2014).A 200-Year Record of Polycyclic Aromatic Hydrocarbons Contamination in an Ombrotrophic Peatland in Great Hinggan Mountain, Northeast China.Journal of Mountain Science,11(5),1085-1096.
MLA	BAO Kun-shan,et al."A 200-Year Record of Polycyclic Aromatic Hydrocarbons Contamination in an Ombrotrophic Peatland in Great Hinggan Mountain, Northeast China".Journal of Mountain Science 11.5(2014):1085-1096.