Polyamorphic transitions in Ce-based metallic glasses by synchrotron radiation | |
Duarte, MJ ; Bruna, P ; Pineda, E ; Crespo, D ; Garbarino, G ; Verbeni, R ; Zhao, K ; Wang, WH ; Romero, AH ; Serrano, J | |
刊名 | PHYSICAL REVIEW B
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2011 | |
卷号 | 84期号:22 |
关键词 | LIQUID PHASE-TRANSITION HIGH-PRESSURE DENSITY SILICON SYSTEMS CERIUM |
ISSN号 | 1098-0121 |
通讯作者 | Duarte, MJ (reprint author), Univ Politecn Cataluna, EPSC, Dept Fis Aplicada, ICREA, C Esteve Terradas 15, E-08860 Castelldefels, Spain. |
中文摘要 | We report here on a polyamorphic-phase transition upon application of pressure on a Ce-based metallic glass, Ce(70)Al(10)Ni(10)Cu(10), investigated by x-ray diffraction and inelastic x-ray scattering. This alloy is found to display a strong hysteresis in volume per atom upon application and subsequent release of pressure. The observed structural changes are correlated with changes observed by inelastic x-ray scattering in the elastic constants, acoustic mode frequencies, and sound speed. The results reported here point toward three different amorphous phases for this alloy existing in the 0-25 GPa pressure region: low-and high-density states and an intermediate mixed state that displays a hysteresis behavior. Finally, we discuss the impact of Ce concentration on the polyamorphic transition for a series of Ce-based metallic glass alloys and link it to the phase transformation between gamma-Ce and alpha-Ce under pressure. |
收录类别 | SCI |
资助信息 | CICYT [MAT2010-14907]; Generalitat de Catalunya [2009SGR1225, 2009SGR1251]; Conacyt, Mexico [152153]; NSF of China [50921091, 50731008]; MOST973 of China [2007CB613904, 2010CB731603] |
语种 | 英语 |
公开日期 | 2013-09-24 |
内容类型 | 期刊论文 |
源URL | [http://ir.iphy.ac.cn/handle/311004/51131] ![]() |
专题 | 物理研究所_物理所公开发表论文_物理所公开发表论文_期刊论文 |
推荐引用方式 GB/T 7714 | Duarte, MJ,Bruna, P,Pineda, E,et al. Polyamorphic transitions in Ce-based metallic glasses by synchrotron radiation[J]. PHYSICAL REVIEW B,2011,84(22). |
APA | Duarte, MJ.,Bruna, P.,Pineda, E.,Crespo, D.,Garbarino, G.,...&Serrano, J.(2011).Polyamorphic transitions in Ce-based metallic glasses by synchrotron radiation.PHYSICAL REVIEW B,84(22). |
MLA | Duarte, MJ,et al."Polyamorphic transitions in Ce-based metallic glasses by synchrotron radiation".PHYSICAL REVIEW B 84.22(2011). |
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