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Valley-selective circular dichroism of monolayer molybdenum disulphide
Cao, T ; Wang, G ; Han, WP ; Ye, HQ ; Zhu, CR ; Shi, JR ; Niu, Q ; Tan, PH ; Wang, E ; Liu, BL ; Feng, J
刊名NATURE COMMUNICATIONS
2012
卷号3
关键词GRAPHENE MOS2
ISSN号2041-1723
通讯作者Feng, J (reprint author), Peking Univ, Int Ctr Quantum Mat, Beijing 100871, Peoples R China.
中文摘要A two-dimensional honeycomb lattice harbours a pair of inequivalent valleys in the k-space electronic structure, in the vicinities of the vertices of a hexagonal Brillouin zone, K-+/-. It is particularly appealing to exploit this emergent degree of freedom of charge carriers, in what is termed 'valleytronics'. The physics of valleys mimics that of spin, and will make possible devices, analogous to spintronics, such as valley filter and valve, and optoelectronic Hall devices, all very promising for next-generation electronics. The key challenge lies with achieving valley polarization, of which a convincing demonstration in a two-dimensional honeycomb structure remains evasive. Here we show, using first principles calculations, that monolayer molybdenum disulphide is an ideal material for valleytronics, for which valley polarization is achievable via valley-selective circular dichroism arising from its unique symmetry. We also provide experimental evidence by measuring the circularly polarized photoluminescence on monolayer molybdenum disulphide, which shows up to 50% polarization.
收录类别SCI
资助信息National Science Foundation of China (NSFC) [11174009, 10974238, 91021007, 11174338, 10934007, 10911130356, 10874177]; National Basic Research Program of China (973 Program) [2009CB929301, 2009CB930500, 2011CBA00109, 2012CB921300]; Welch Foundation [F-1255]; DOE-DMSE [DE-FG03-02ER45958]
语种英语
公开日期2013-09-23
内容类型期刊论文
源URL[http://ir.iphy.ac.cn/handle/311004/46492]  
专题物理研究所_物理所公开发表论文_物理所公开发表论文_期刊论文
推荐引用方式
GB/T 7714
Cao, T,Wang, G,Han, WP,et al. Valley-selective circular dichroism of monolayer molybdenum disulphide[J]. NATURE COMMUNICATIONS,2012,3.
APA Cao, T.,Wang, G.,Han, WP.,Ye, HQ.,Zhu, CR.,...&Feng, J.(2012).Valley-selective circular dichroism of monolayer molybdenum disulphide.NATURE COMMUNICATIONS,3.
MLA Cao, T,et al."Valley-selective circular dichroism of monolayer molybdenum disulphide".NATURE COMMUNICATIONS 3(2012).
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