High contribution of anthropogenic combustion sources to atmosphericinorganic reactive nitrogen in South China evidenced by isotopes

doi:10.5194/acp-23-6395-2023

CORC > 烟台海岸带研究所 > 中国科学院烟台海岸带研究所 > 中科院海岸带环境过程与生态修复重点实验室

	High contribution of anthropogenic combustion sources to atmosphericinorganic reactive nitrogen in South China evidenced by isotopes
	Li, Tingting 1,2,4,5; Li, Jun 1,4,5; Sun, Zeyu 2,3; Jiang, Hongxing 1,5; Tian, Chongguo 3; Zhang, Gan 1,4,5
刊名	ATMOSPHERIC CHEMISTRY AND PHYSICS
	2023-06-12
卷号	23 期号:11 页码:6395-6407
ISSN号	1680-7316
DOI	10.5194/acp-23-6395-2023
通讯作者	Li, Jun(junli@gig.ac.cn)
英文摘要	Due to the intense release of reactive nitrogen (Nr) from anthropogenic activity, the source layout of atmospheric nitrogen aerosol has changed. To comprehensively clarify the level, sources, and environmental fate of NH4+ and NO3- , their concentrations and stable isotopes (d(15)N) in fine particulate matter (PM2.5) were measured in a subtropical megacity of South China. The inorganic nitrogen (NH4+ and NO3-) was an essential part of atmospheric nitrogen aerosol, and the N-NH4+ and N-NO3- contributed 45.8 % and 23.2 % to total nitrogen (TN), respectively. The source contributions of NH4+ and NO3- were estimated by d(15)N, suggesting that the dominant sources were from anthropogenic combustion activities, including coal combustion, biomass burning, and vehicles, contributing 63.2 % and 88.3 % to NH4+ and NO3- , respectively. In particular, biomass burning was the predominant source of NH4+ (27.9 %), whereas coal combustion was the dominant source of NO3- (40.4 %). This study emphasized the substantial impacts of human activities on inorganic Nr. With the rapid development of industry and transportation, nitrogen emissions will be even higher. The promotion of clean energy and efficient use of biomass would help to reduce nitrogen emissions and alleviate air pollution.
WOS关键词	SOURCE APPORTIONMENT ; TROPOSPHERIC OZONE ; EMISSION SOURCES ; AIR-QUALITY ; NOX ; AMMONIA ; NITRATE ; AEROSOL ; DEPOSITION ; PRECIPITATION
WOS研究方向	Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
语种	英语
WOS记录号	WOS:001006668100001
资助机构	Natural Science Foundation of China (NSFC) ; Basic and Applied Basic Research Foundation of Guangdong Province ; Guangdong Science and Technology Innovation Foundation
内容类型	期刊论文
源URL	[http://ir.yic.ac.cn/handle/133337/33309]
专题	烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
通讯作者	Li, Jun
作者单位	1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Key Lab Environm Protect & Resources Utilizat, Guangzhou 510640, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China 4.Chinese Acad Sci, Ctr Excellence Deep Earth Sci, Guangzhou 510640, Peoples R China 5.Chinese Acad Sci, Guangzhou Inst Geochem, Guangdong Hong Kong Macao Joint Lab Environm Pollu, Guangzhou 510640, Peoples R China
推荐引用方式 GB/T 7714	Li, Tingting,Li, Jun,Sun, Zeyu,et al. High contribution of anthropogenic combustion sources to atmosphericinorganic reactive nitrogen in South China evidenced by isotopes[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2023,23(11):6395-6407.
APA	Li, Tingting,Li, Jun,Sun, Zeyu,Jiang, Hongxing,Tian, Chongguo,&Zhang, Gan.(2023).High contribution of anthropogenic combustion sources to atmosphericinorganic reactive nitrogen in South China evidenced by isotopes.ATMOSPHERIC CHEMISTRY AND PHYSICS,23(11),6395-6407.
MLA	Li, Tingting,et al."High contribution of anthropogenic combustion sources to atmosphericinorganic reactive nitrogen in South China evidenced by isotopes".ATMOSPHERIC CHEMISTRY AND PHYSICS 23.11(2023):6395-6407.