Heavy metal mobility in contaminated sediments under seawater acidification
Gao, Wenjing4; Qu, Baoxiao1,2,3; Yuan, Huamao1,2,3; Song, Jinming1,2,3; Li, Weibing4
刊名MARINE POLLUTION BULLETIN
2023-07-01
卷号192页码:5
关键词Heavy metals Ocean acidification Sediment pH leaching experiment Mobility
ISSN号0025-326X
DOI10.1016/j.marpolbul.2023.115062
通讯作者Qu, Baoxiao(qubx@qdio.ac.cn) ; Yuan, Huamao(yuanhuamao@qdio.ac.cn)
英文摘要The behavior of heavy metals in contaminated sediment is of ecological significance considering the change of pH caused by ocean acidification. This study investigated the mobility of Cd, Cu, Ni, Pb, Fe, and Mn under experimental conditions for seawater acidification via enrichment of CO2 gas at different reaction set-ups. The results indicated that the concerned metals behaved differently in the water compared to the sediment. The heavy metals were considerably transferred from sediment to seawater, and the resultant intensity was controlled by the degree of acidification and the chemical state of specific metals. Moreover, labile fractions of heavy metals in sediments were more susceptible to acidification than other fractions. These findings were observed and confirmed using real-time monitoring conducted via the diffusion gradient technique (DGT). Overall, the results of this study provided new insights into exploring the coupling risk of heavy metals with ocean acidification.
资助项目National Natural Science Foundation of China[42276206] ; National Natural Science Foundation of China[41976037] ; National Natural Science Foundation of China[41806133] ; Taishan Scholars Program ; Shandong Provincial Natural Science Foundation[ZR2020YQ28]
WOS关键词SURFACE SEDIMENTS ; JIAOZHOU BAY ; POLLUTION STATUS ; RISK-ASSESSMENT ; RELEASE ; SPECIATION ; CO2 ; PH ; FRACTIONATION ; OXIDATION
WOS研究方向Environmental Sciences & Ecology ; Marine & Freshwater Biology
语种英语
出版者PERGAMON-ELSEVIER SCIENCE LTD
WOS记录号WOS:001007131600001
内容类型期刊论文
源URL[http://ir.qdio.ac.cn/handle/337002/182261]  
专题海洋研究所_海洋生态与环境科学重点实验室
通讯作者Qu, Baoxiao; Yuan, Huamao
作者单位1.Chinese Acad Sci, Ctr Ocean Mega Sci, Qingdao 266071, Peoples R China
2.Qingdao Natl Lab Marine Sci & Technol, Lab Marine Ecol & Environm Sci, Qingdao 266237, Peoples R China
3.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Ecol & Environm Sci, Qingdao 266071, Peoples R China
4.Qingdao Univ Sci & Technol, Coll Environm & Safety Engn, Qingdao 266042, Peoples R China
推荐引用方式
GB/T 7714
Gao, Wenjing,Qu, Baoxiao,Yuan, Huamao,et al. Heavy metal mobility in contaminated sediments under seawater acidification[J]. MARINE POLLUTION BULLETIN,2023,192:5.
APA Gao, Wenjing,Qu, Baoxiao,Yuan, Huamao,Song, Jinming,&Li, Weibing.(2023).Heavy metal mobility in contaminated sediments under seawater acidification.MARINE POLLUTION BULLETIN,192,5.
MLA Gao, Wenjing,et al."Heavy metal mobility in contaminated sediments under seawater acidification".MARINE POLLUTION BULLETIN 192(2023):5.
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