High-order harmonics generation in nanosecond-pulses-induced plasma containing Ni-doped CsPbBr3 perovskite nanocrystals using chirp-free and chirped femtosecond pulses
S. R. Konda; R. A. Ganeev; V. V. Kim; R. Ketavath; J. Q. Yu and W. Li
刊名Nanotechnology
2023
卷号34期号:5页码:13
ISSN号0957-4484
DOI10.1088/1361-6528/ac9fdb
英文摘要We demonstrate high-order harmonic generation in Ni-doped CsPbBr3 perovskite nanocrystals ablated by nanosecond pulses using chirp-free 35 fs, and chirped 135 fs pulses in the case of single-color pump (800 nm) and a two-color pump (800 and 400 nm). We analyzed the spectral shift, cut-off, and intensity distribution of harmonics in the case of chirped drving pulses compared to chirp-free pulses. It is shown that the presence of Ni dopants and CsPbBr3 plasma components improves the harmonics emission. Also, we measured the third-order nonlinear optical (NLO) properties of these nanocrystals using 800 nm, 60 fs, 1 kHz pulses. The variations of measured NLO parameters of CsPbBr3 perovskite nanocrystals containing different concentrations of nickel correlate with variations of generated high-order harmonics from laser induced plasmas of studied nanocrystals in terms of harmonics intensity, cut-off, and spectral shift (in case of chirped driving pulses). The spectral shift of the harmonics generated from the Ni-doped CsPbBr3 perovskite nanocrystals can be used to form tunable extreme ultraviolet sources.
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语种英语
内容类型期刊论文
源URL[http://ir.ciomp.ac.cn/handle/181722/66716]  
专题中国科学院长春光学精密机械与物理研究所
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S. R. Konda,R. A. Ganeev,V. V. Kim,et al. High-order harmonics generation in nanosecond-pulses-induced plasma containing Ni-doped CsPbBr3 perovskite nanocrystals using chirp-free and chirped femtosecond pulses[J]. Nanotechnology,2023,34(5):13.
APA S. R. Konda,R. A. Ganeev,V. V. Kim,R. Ketavath,&J. Q. Yu and W. Li.(2023).High-order harmonics generation in nanosecond-pulses-induced plasma containing Ni-doped CsPbBr3 perovskite nanocrystals using chirp-free and chirped femtosecond pulses.Nanotechnology,34(5),13.
MLA S. R. Konda,et al."High-order harmonics generation in nanosecond-pulses-induced plasma containing Ni-doped CsPbBr3 perovskite nanocrystals using chirp-free and chirped femtosecond pulses".Nanotechnology 34.5(2023):13.
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