Understanding composition-dependent catalytic performance of PdAg for the hydrogenation of 1,3-butadiene to 1-butene

doi:10.1016/j.catcom.2020.106255

	Understanding composition-dependent catalytic performance of PdAg for the hydrogenation of 1,3-butadiene to 1-butene
	Ma, Haowen 1,2; Xu, Xiaopei 3; Xu, Haoxiang 3; Feng, Huixia 2; Xie, Yuan 1; Cheng, Daojian 3
刊名	Catalysis Communications
	2021-01-15
卷号	149
关键词	Binary alloys Butenes Density functional theory Hydrogenation Palladium alloys Silver 1-butene Ag catalysts Bimetallic surfaces Binding strength Catalytic performance Catalytic properties Hydrogenation of 1 ,3 butadienes Partial hydrogenation
ISSN号	15667367
DOI	10.1016/j.catcom.2020.106255
英文摘要	The composition-dependent adsorption and catalytic properties of Pd–Ag bimetallic surfaces for the partial hydrogenation of 1,3-butadiene to 1-butene were studied by density functional theory. With the increase of Ag content, the activity and selectivity for the partial hydrogenation of 1,3-butadiene to 1-butene were enhanced with the decrease in binding strength of adsorbates. The increase of surface Ag content in Pd–Ag catalysts can thus enhance the catalytic performance of the hydrogenation of 1,3-butadiene. © 2020 The Authors
WOS研究方向	Chemistry
语种	英语
出版者	Elsevier B.V.
WOS记录号	WOS:000600589400058
内容类型	期刊论文
源URL	[http://ir.lut.edu.cn/handle/2XXMBERH/147159]
专题	教务处（创新创业学院）
作者单位	1.Lanzhou Petrochemical Research Center of PetroChina, LanZhou; 730000, China 2.College of Petrochemical Technology, State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals, Lanzhou University of Technology, LanZhou; 730000, China; 3.State Key Laboratory of Organic-Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, Beijing University of Chemical Technology, Beijing; 100029, China;
推荐引用方式 GB/T 7714	Ma, Haowen,Xu, Xiaopei,Xu, Haoxiang,et al. Understanding composition-dependent catalytic performance of PdAg for the hydrogenation of 1,3-butadiene to 1-butene[J]. Catalysis Communications,2021,149.
APA	Ma, Haowen,Xu, Xiaopei,Xu, Haoxiang,Feng, Huixia,Xie, Yuan,&Cheng, Daojian.(2021).Understanding composition-dependent catalytic performance of PdAg for the hydrogenation of 1,3-butadiene to 1-butene.Catalysis Communications,149.
MLA	Ma, Haowen,et al."Understanding composition-dependent catalytic performance of PdAg for the hydrogenation of 1,3-butadiene to 1-butene".Catalysis Communications 149(2021).