Single-Atom Catalysts for the Electrocatalytic Reduction of Nitrogen to Ammonia under Ambient Conditions

doi:10.1002/asia.201900793

CORC > 兰州理工大学 > 兰州理工大学 > 省部共建有色金属先进加工与再利用国家重点实验室

	Single-Atom Catalysts for the Electrocatalytic Reduction of Nitrogen to Ammonia under Ambient Conditions
	Qiu, Yuan 1,4; Peng, Xianyun 1,4; Lue, Fang 1,4; Mi, Yuying 1,4; Zhuo, Longchao 3; Ren, Junqiang 2; Liu, Xijun 1,4; Luo, Jun 1,4
刊名	CHEMISTRY-AN ASIAN JOURNAL
	2019-07-26
卷号	14 期号:16 页码:2770-2779
关键词	ambient conditions ammonia synthesis electrochemistry nitrogen fixation single-atom catalysts
ISSN号	1861-4728
DOI	10.1002/asia.201900793
英文摘要	Powered by renewable electricity, the electrochemical reduction of nitrogen to ammonia is proposed as a promising alternative to the energy- and capital-intensive Haber-Bosch process, and has thus attracted much attention from the scientific community. However, this process suffers from low NH3 yields and Faradaic efficiency. The development of more effective electrocatalysts is of vital importance for the practical applications of this reaction. Of the reported catalysts, single-atom catalysts (SACs) show the significant advantages of efficient atom utilization and unsaturated coordination configurations, which offer great scope for optimizing their catalytic performance. Herein, progress in state-of-the-art SACs applied in the electrocatalytic N-2 reduction reaction (NRR) is discussed, and the main advantages and challenges for developing more efficient electrocatalysts are also highlighted.
资助项目	Science & Technology Development Fund of Tianjin Education Commission for Higher Education[2018KJ126]
WOS研究方向	Chemistry
语种	英语
出版者	WILEY-V C H VERLAG GMBH
WOS记录号	WOS:000478483200001
状态	已发表
内容类型	期刊论文
源URL	[http://119.78.100.223/handle/2XXMBERH/31708]
专题	省部共建有色金属先进加工与再利用国家重点实验室
通讯作者	Liu, Xijun
作者单位	1.Tianjin Univ Technol, Sch Mat Sci & Engn, Inst New Energy Mat & Low Carbon Technol, Tianjin Key Lab Adv Funct Porous Mat, Tianjin 300384, Peoples R China 2.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Lanzhou 730050, Gansu, Peoples R China 3.Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China 4.Tianjin Univ Technol, Sch Mat Sci & Engn, Inst New Energy Mat & Low Carbon Technol, Ctr Electron Microscopy, Tianjin 300384, Peoples R China
推荐引用方式 GB/T 7714	Qiu, Yuan,Peng, Xianyun,Lue, Fang,et al. Single-Atom Catalysts for the Electrocatalytic Reduction of Nitrogen to Ammonia under Ambient Conditions[J]. CHEMISTRY-AN ASIAN JOURNAL,2019,14(16):2770-2779.
APA	Qiu, Yuan.,Peng, Xianyun.,Lue, Fang.,Mi, Yuying.,Zhuo, Longchao.,...&Luo, Jun.(2019).Single-Atom Catalysts for the Electrocatalytic Reduction of Nitrogen to Ammonia under Ambient Conditions.CHEMISTRY-AN ASIAN JOURNAL,14(16),2770-2779.
MLA	Qiu, Yuan,et al."Single-Atom Catalysts for the Electrocatalytic Reduction of Nitrogen to Ammonia under Ambient Conditions".CHEMISTRY-AN ASIAN JOURNAL 14.16(2019):2770-2779.