Single-Atom Catalysts for the Electrocatalytic Reduction of Nitrogen to Ammonia under Ambient Conditions

doi:10.1002/asia.201900793

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	Single-Atom Catalysts for the Electrocatalytic Reduction of Nitrogen to Ammonia under Ambient Conditions
	Qiu, Yuan 3; Peng, Xianyun 3; Lü, Fang 3; Mi, Yuying 3; Zhuo, Longchao 2; Ren, Junqiang 1; Liu, Xijun 3; Luo, Jun 3
刊名	Chemistry - An Asian Journal
	2019
卷号	14 期号:16 页码:2770-2779
关键词	Ammonia Atoms Electrocatalysts Electrochemistry Electrolytic reduction
ISSN号	18614728
DOI	10.1002/asia.201900793
英文摘要	Powered by renewable electricity, the electrochemical reduction of nitrogen to ammonia is proposed as a promising alternative to the energy- and capital-intensive Haber–Bosch process, and has thus attracted much attention from the scientific community. However, this process suffers from low NH3 yields and Faradaic efficiency. The development of more effective electrocatalysts is of vital importance for the practical applications of this reaction. Of the reported catalysts, single-atom catalysts (SACs) show the significant advantages of efficient atom utilization and unsaturated coordination configurations, which offer great scope for optimizing their catalytic performance. Herein, progress in state-of-the-art SACs applied in the electrocatalytic N2 reduction reaction (NRR) is discussed, and the main advantages and challenges for developing more efficient electrocatalysts are also highlighted. © 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim
WOS研究方向	Chemistry
语种	英语
出版者	John Wiley and Sons Ltd
WOS记录号	WOS:000478483200001
内容类型	期刊论文
源URL	[http://ir.lut.edu.cn/handle/2XXMBERH/151194]
专题	省部共建有色金属先进加工与再利用国家重点实验室继续教育学院
作者单位	1.State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals, Lanzhou University of Technology, Lanzhou; 730050, China 2.School of Materials Science and Engineering, Xi'an University of Technology, Xi'an; 710048, China; 3.Center for Electron Microscopy and Tianjin Key Lab of Advanced Functional Porous Materials, Institute for New Energy Materials and Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of Technology, Tianjin; 300384, China;
推荐引用方式 GB/T 7714	Qiu, Yuan,Peng, Xianyun,Lü, Fang,et al. Single-Atom Catalysts for the Electrocatalytic Reduction of Nitrogen to Ammonia under Ambient Conditions[J]. Chemistry - An Asian Journal,2019,14(16):2770-2779.
APA	Qiu, Yuan.,Peng, Xianyun.,Lü, Fang.,Mi, Yuying.,Zhuo, Longchao.,...&Luo, Jun.(2019).Single-Atom Catalysts for the Electrocatalytic Reduction of Nitrogen to Ammonia under Ambient Conditions.Chemistry - An Asian Journal,14(16),2770-2779.
MLA	Qiu, Yuan,et al."Single-Atom Catalysts for the Electrocatalytic Reduction of Nitrogen to Ammonia under Ambient Conditions".Chemistry - An Asian Journal 14.16(2019):2770-2779.