Fabrication of Au–Pd NPs@CNSs/GO Nanocomposites and Their High Catalytic Properties | |
Ce Su; Huang, Xuelian; Wang, Qili; Shang, Zhaoyang; Wei, Yunbiao; Li, Guanbin; Li, Siliang | |
刊名 | Russian Journal of Physical Chemistry A |
2020-09-01 | |
卷号 | 94期号:9页码:1804-1810 |
关键词 | Aromatic compounds Ascorbic acid Catalyst selectivity Degradation Fabrication Graphene Nanocomposites Nanospheres Palladium alloys Sodium Borohydride Carbon nanosphere Catalytic properties Degradation efficiency Diethylenetriamine In-situ growth Particle diameters PD nano particle Selective degradation |
ISSN号 | 00360244 |
DOI | 10.1134/S0036024420090277 |
英文摘要 | Abstract: Au–Pd NPs@CNSs/GO nanocomposites have been fabricated by the in situ growth of Au–Pd nanoparticles on carbon nanospheres (CNSs) using ascorbic acid as reducing agent and diethylenetriamine (DETA) as a coupling linker and the subsequent assembly of the Au–Pd NPs@CNSs on graphene oxide (GO). In the nanocomposites, the Au–Pd NPs alloys have an average particle diameter of less than 10 nm. The nanocomposites show excellent catalytic activity for methylene blue with a high degradation efficiency above 99% in the presence of NaBH4 in aqueous solution, which is attributed to the effects of Au–Pd NPs alloys in the nanocomposites. In addition, the catalyst exhibits good selectivity for methylene blue in the presence of other organic dyes. Meanwhile, the catalytic activity remains unchanged for nine cycles. Such features ensure a very promising application of nanocomposites in the selective degradation of methylene blue in dyes mixtures. © 2020, Pleiades Publishing, Ltd. |
WOS研究方向 | Chemistry |
语种 | 英语 |
出版者 | Pleiades Publishing |
WOS记录号 | WOS:000566344200011 |
内容类型 | 期刊论文 |
源URL | [http://ir.lut.edu.cn/handle/2XXMBERH/115124] |
专题 | 石油化工学院 |
作者单位 | School of Petrochemical Engineering, Lanzhou University of Technology, Lanzhou; 730050, China |
推荐引用方式 GB/T 7714 | Ce Su,Huang, Xuelian,Wang, Qili,et al. Fabrication of Au–Pd NPs@CNSs/GO Nanocomposites and Their High Catalytic Properties[J]. Russian Journal of Physical Chemistry A,2020,94(9):1804-1810. |
APA | Ce Su.,Huang, Xuelian.,Wang, Qili.,Shang, Zhaoyang.,Wei, Yunbiao.,...&Li, Siliang.(2020).Fabrication of Au–Pd NPs@CNSs/GO Nanocomposites and Their High Catalytic Properties.Russian Journal of Physical Chemistry A,94(9),1804-1810. |
MLA | Ce Su,et al."Fabrication of Au–Pd NPs@CNSs/GO Nanocomposites and Their High Catalytic Properties".Russian Journal of Physical Chemistry A 94.9(2020):1804-1810. |
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