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Creating a new electrode material of supercapacitors from the waste multi-walled carbon nanotubes
Chen, Yong; Xu, Cheng; Zhao, Jiang; Huang, Jiandi; Xu, Hui; Gou, Guojun
刊名ELECTROCHIMICA ACTA
2020-01-10
卷号330
关键词Adsorption Waste MWCNTs MWCNTs/MB/PPy composites Specific capacitance Symmetric supercapacitor
ISSN号0013-4686
DOI10.1016/j.electacta.2019.135237
英文摘要Many adsorbents are discarded after removing pollutants, which always re-contaminateenvironment due to a release of pollutants again. The purpose of this study is to reuse the waste multi-walled carbon nanotubes (MWCNTs) who remove methylene blue (MB) from waste water as electrode material of supercapacitor. Herein, with a combination of polypyrrole (PPy), MWCNTs/MB/PPy composites are synthesized via chemical in-situ polymerization. The structure tests of the composites indicate that the surface property of MWCNTs, after adsorbing MB, is changed from hydrophobic to hydrophilic. Additionally, cyclic voltammetry (CV), galvanostatic charge-discharge (GCD), and electrochemical impedance spectrum (EIS) tests in three-electrode system demonstrate that at a current density of 5 mA cm(-2), the specific capacitance of MWCNTs/MB/PPy composites is 446 F g(-1). This result is higher than that of PPy and MWCNTs/PPy composites due to an extra pseudo-capacitance provided by MB. Moreover, a symmetric supercapacitor of MWCNTs/MB/PPy composites is assembled to successfully light a light emitting diodes (LED), which powerfully reveals the potential application of MWCNTs/MB/PPy composites. Obviously, the waste MWCNTs can be reused, meaning the dyes adsorbed on MWCNTs have no chance to pollute the environment again. (C) 2019 Elsevier Ltd. All rights reserved.
资助项目National Natural Science Foundations of China[51663014][51503092][51763015] ; Natural Science Foundation of Gansu Province[2017GS10857]
WOS研究方向Electrochemistry
语种英语
出版者PERGAMON-ELSEVIER SCIENCE LTD
WOS记录号WOS:000501468400018
状态已发表
内容类型期刊论文
源URL[http://ir.lut.edu.cn/handle/2XXMBERH/64235]  
专题石油化工学院
通讯作者Chen, Yong; Xu, Hui
作者单位Lanzhou Univ Technol, Coll Petrochem Engn, Lanzhou 730050, Gansu, Peoples R China
推荐引用方式
GB/T 7714
Chen, Yong,Xu, Cheng,Zhao, Jiang,et al. Creating a new electrode material of supercapacitors from the waste multi-walled carbon nanotubes[J]. ELECTROCHIMICA ACTA,2020,330.
APA Chen, Yong,Xu, Cheng,Zhao, Jiang,Huang, Jiandi,Xu, Hui,&Gou, Guojun.(2020).Creating a new electrode material of supercapacitors from the waste multi-walled carbon nanotubes.ELECTROCHIMICA ACTA,330.
MLA Chen, Yong,et al."Creating a new electrode material of supercapacitors from the waste multi-walled carbon nanotubes".ELECTROCHIMICA ACTA 330(2020).
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