Engineering MOFs-Derived Nanoarchitectures with Efficient Polysulfides Catalytic Sites for Advanced Li-S Batteries

doi:10.1002/admt.202200238

	Engineering MOFs-Derived Nanoarchitectures with Efficient Polysulfides Catalytic Sites for Advanced Li-S Batteries
	Tao, Xuefeng 1; Yang, Zhao 3; Yan, Rui 1; Cheng, Menghao 1; Ma, Tian 1; Cao, Sujiao 1; Bai, Mingru 1; Ran, Fen 3; Cheng, Chong 1,2; Yang, Wei 1
刊名	ADVANCED MATERIALS TECHNOLOGIES
	2022-07-01
关键词	energy-storage materials lithium-sulfur batteries metal-organic frameworks nanoarchitecture polysulfides catalysts
ISSN号	2365-709X
DOI	10.1002/admt.202200238
英文摘要	Lithium-sulfur batteries (LSBs) have received dramatically increased attention because of their manifest advantages. Nevertheless, due to the severe shuttling of lithium polysulfides (LiPSs), sluggish reaction kinetics, and the insulation of sulfur species, the practical application of LSBs is far away. To overcome the abovementioned issues, metal-organic frameworks (MOFs)-derived nanoarchitectures have emerged as one of the most promising cathode materials in designing advanced Li-S batteries. This timely progress report highlights and comments on the most recent advances in designing MOFs-derived nanoarchitectures with diverse electrocatalytic centers as cathode materials for catalyzing the oxidation/reduction reactions of LiPS in LSBs. The molecular/atomic-level electrocatalytic centers, tunable porosities, large specific surface area, controlled components, and versatile structures of MOFs-derived nanoarchitectures are carefully discussed for designing favorable electrocatalysts for LiPS. In particular, the catalytic mechanisms of LiPS based on different types of MOFs-derived materials ranging from single atoms to nanoparticles are systematically summarized. Ultimately, the prospects and challenges of engineering MOFs-derived catalysts for LiPS in LSBs are also suggested. It is believed that this progress report will offer potential guidance and instructive perspectives for designing future state-of-the-art LiPS catalytic materials in LSBs.
WOS研究方向	Materials Science
语种	英语
出版者	WILEY
WOS记录号	WOS:000819971900001
内容类型	期刊论文
源URL	[http://ir.lut.edu.cn/handle/2XXMBERH/158934]
专题	材料科学与工程学院
作者单位	1.Sichuan Univ, Coll Polymer Sci & Engn, State Key Lab Polymer Mat Engn, Chengdu 610065, Peoples R China; 2.Free Univ Berlin, Dept Chem & Biochem, Takustr 3, D-14195 Berlin, Germany 3.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Lanzhou 730050, Gansu, Peoples R China;
推荐引用方式 GB/T 7714	Tao, Xuefeng,Yang, Zhao,Yan, Rui,et al. Engineering MOFs-Derived Nanoarchitectures with Efficient Polysulfides Catalytic Sites for Advanced Li-S Batteries[J]. ADVANCED MATERIALS TECHNOLOGIES,2022.
APA	Tao, Xuefeng.,Yang, Zhao.,Yan, Rui.,Cheng, Menghao.,Ma, Tian.,...&Yang, Wei.(2022).Engineering MOFs-Derived Nanoarchitectures with Efficient Polysulfides Catalytic Sites for Advanced Li-S Batteries.ADVANCED MATERIALS TECHNOLOGIES.
MLA	Tao, Xuefeng,et al."Engineering MOFs-Derived Nanoarchitectures with Efficient Polysulfides Catalytic Sites for Advanced Li-S Batteries".ADVANCED MATERIALS TECHNOLOGIES (2022).