Atomic mapping of structural distortions in 109 degrees domain patterned BiFeO3 thin films | |
Wang, Wen-Yuan1,2; Zhu, Yin-Lian1; Tang, Yun-Long1; Han, Meng-Jiao1; Wang, Yu-Jia1; Ma, Xiu-Liang1,3 | |
刊名 | JOURNAL OF MATERIALS RESEARCH |
2017-06 | |
卷号 | 32期号:12页码:2423-2430 |
ISSN号 | 0884-2914 |
DOI | 10.1557/jmr.2017.206 |
英文摘要 | Structural distortions at the nanoscale are delicately linked with many exotic properties for ferroic thin films. Based on advanced aberration corrected scanning transmission electron microscopy, we observe BiFeO3 thin films with variant tensile strain states and demonstrate at an atomic scale the interplay of intrinsic spontaneous structural distortions with external constraints. Structural parameters (the rhombohedral distortion and domain wall shear distortion) under zero (BiFeO3/GdScO3) and 1.5% (BiFeO3/PrScO3) lateral strain states are quantitatively analyzed which are suppressed within a few unit cells near the film/substrate interfaces. In particular, an interfacial layer with asymmetrical lattice distortions (enhanced and reduced out-of-plane lattice spacing) on the two sides of 109 degrees domain wall is resolved. These structural distortions near the film/substrate interface in ferroic thin films reveal intense tanglement of intrinsic distortions of BiFeO3 with external boundary conditions, which could provide new insights for the development of nanoscale ferroelectric devices. |
资助项目 | Key Research Program of Frontier Sciences, CAS[QYZDJ-SSW-JSC010] |
WOS研究方向 | Materials Science |
语种 | 英语 |
出版者 | CAMBRIDGE UNIV PRESS |
WOS记录号 | WOS:000404965300023 |
状态 | 已发表 |
内容类型 | 期刊论文 |
源URL | [http://119.78.100.223/handle/2XXMBERH/33257] |
专题 | 材料科学与工程学院 材料科学与工程学院_特聘教授组 |
通讯作者 | Ma, Xiu-Liang |
作者单位 | 1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China 2.Sci & Technol Surface Phys & Chem Lab, Jiangyou 621908, Sichuan, Peoples R China 3.Lanzhou Univ Technol, Sch Mat Sci & Engn, Lanzhou 730050, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Wen-Yuan,Zhu, Yin-Lian,Tang, Yun-Long,et al. Atomic mapping of structural distortions in 109 degrees domain patterned BiFeO3 thin films[J]. JOURNAL OF MATERIALS RESEARCH,2017,32(12):2423-2430. |
APA | Wang, Wen-Yuan,Zhu, Yin-Lian,Tang, Yun-Long,Han, Meng-Jiao,Wang, Yu-Jia,&Ma, Xiu-Liang.(2017).Atomic mapping of structural distortions in 109 degrees domain patterned BiFeO3 thin films.JOURNAL OF MATERIALS RESEARCH,32(12),2423-2430. |
MLA | Wang, Wen-Yuan,et al."Atomic mapping of structural distortions in 109 degrees domain patterned BiFeO3 thin films".JOURNAL OF MATERIALS RESEARCH 32.12(2017):2423-2430. |
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