Photoinduced interlayer dynamics in T-d-MoTe2: A broadband pump-probe study | |
Cheng, Meixin1,2; Zhong, Shazhou3,4; Rivas, Nicolas1,2,8; Dekker, Tina3,4; Petruk, Ariel Alcides1,2; Gicala, Patrick1,2; Pichugin, Kostyantyn1,2; Chen, Fangchu3,4; Luo, Xuan5; Sun, Yuping5,6,7 | |
刊名 | APPLIED PHYSICS LETTERS |
2022-03-21 | |
卷号 | 120 |
ISSN号 | 0003-6951 |
DOI | 10.1063/5.0084986 |
通讯作者 | Sciaini, German(gsciaini@uwaterloo.ca) |
英文摘要 | We report on time-resolved broadband transient reflectivity (tr-bb-TR) measurements performed on a bulk single crystal of T-d-MoTe2 as a function of the incident pump fluence (F). Tr-bb-TR data unveil photoinduced electronic changes progressing on the sub-picosecond timescale as well as the dynamics of the coherent low-frequency (1)A(1) interlayer shear phonon. Our results indicate a gradual evolution of both the TR and the (1)A(1) Fourier intensity spectra as a function of F, ruling out the threshold-like change that has been associated with the ultrafast photoinduced T-d -> 1T' phase transition. We also observe a large redshift of the (1)A(1) Fourier spectral features, which implies that large renormalization effects are taking place on the interband transitions that are dielectrically susceptible to the (1)A(1) interlayer shear phonon displacement.& nbsp;& nbsp;Published under an exclusive license by AIP Publishing. |
资助项目 | National Research Council of Canada ; Canada Foundation for Innovation ; Canada Research Chair program ; U.S. Army Research Office[W911NF-21-2-0136] ; Ontario Early Researcher Award[ER17-13-199] ; National Science and Engineering Research Council of Canada[RGPIN-2017-03815] ; Canada First Research Excellence Fund ; National Key Research and Development Program[2021YFA1600201] ; National Nature Science Foundation of China[11674326] ; National Nature Science Foundation of China[11874357] ; National Natural Science Foundation of China ; Chinese Academy of Sciences' Large-Scale Scientific Facility[U1832141] ; Chinese Academy of Sciences' Large-Scale Scientific Facility[U1932217] |
WOS关键词 | COHERENT PHONON OSCILLATIONS ; THZ PHONONS ; TRANSITION ; MOTIONS ; PULSES ; MOTE2 ; PHASE |
WOS研究方向 | Physics |
语种 | 英语 |
出版者 | AIP Publishing |
WOS记录号 | WOS:000781898400004 |
资助机构 | National Research Council of Canada ; Canada Foundation for Innovation ; Canada Research Chair program ; U.S. Army Research Office ; Ontario Early Researcher Award ; National Science and Engineering Research Council of Canada ; Canada First Research Excellence Fund ; National Key Research and Development Program ; National Nature Science Foundation of China ; National Natural Science Foundation of China ; Chinese Academy of Sciences' Large-Scale Scientific Facility |
内容类型 | 期刊论文 |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/128447] |
专题 | 中国科学院合肥物质科学研究院 |
通讯作者 | Sciaini, German |
作者单位 | 1.Univ Waterloo, Waterloo Inst Nanotechnol, Waterloo, ON N2L 3G1, Canada 2.Univ Waterloo, Ultrafast Elect Imaging Lab, Dept Chem, Waterloo, ON N2L 3G1, Canada 3.Univ Waterloo, Inst Quantum Comp, Dept Phys & Astron, Dept Elect & Comp Engn, Waterloo, ON N2L 3G1, Canada 4.Univ Waterloo, Dept Chem, Waterloo, ON N2L 3G1, Canada 5.Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, HFIPS, Hefei 230031, Peoples R China 6.Chinese Acad Sci, High Magnet Field Lab, HFIPS, Hefei 230031, Peoples R China 7.Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Peoples R China 8.McMaster Univ, Nucl Engn Grp, Hamilton, ON L8S 4K1, Canada |
推荐引用方式 GB/T 7714 |
Cheng, Meixin,Zhong, Shazhou,Rivas, Nicolas,et al. Photoinduced interlayer dynamics in T-d-MoTe2: A broadband pump-probe study [J]. APPLIED PHYSICS LETTERS,2022,120. |
APA |
Cheng, Meixin.,Zhong, Shazhou.,Rivas, Nicolas.,Dekker, Tina.,Petruk, Ariel Alcides.,...&Sciaini, German.(2022). Photoinduced interlayer dynamics in T-d-MoTe2: A broadband pump-probe study .APPLIED PHYSICS LETTERS,120. |
MLA |
Cheng, Meixin,et al." Photoinduced interlayer dynamics in T-d-MoTe2: A broadband pump-probe study ".APPLIED PHYSICS LETTERS 120(2022). |
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