Ultrasound assisted fabrication of AgBr TiO2 nano-tube arrays photoelectrode and its enhanced visible photocatalytic performance and mechanism for detoxification of 4-chlorphenol
Cui, Yuqi; Zhang, Zixuan; Li, Bo; Guo, Ruonan; Zhang, Xinyi; Cheng, Xiuwen; Xie, Mingzheng; Cheng, Qingfeng
刊名SEPARATION AND PURIFICATION TECHNOLOGY
2018-05-31
卷号197页码:189-196
ISSN号1383-5866
DOI10.1016/j.seppur.2018.01.018
英文摘要In the present work, narrow band gap AgBr nano-particle decorated TiO2 nanotubes arrays (AgBr/TiO2 NTAs) photoelectrode was successfully fabricated through anodization, followed by ultrasonic assisted precipitation process. Subsequently, morphologies and chemical structures were investigated through scanning electron microscope (SEM), X-ray diffraction (XRD) and X-ray photoelectron spectroscopy (XPS). In addition, the optical and photoelectrochemical (PECH) properties were recorded through Ultraviolet-visible diffuse reflectance spectroscopy (UV-vis DRS), transient photocurrent density and Mott-Schottky measurements. Furthermore, the photocatalytic (PC) efficiency was evaluated through the yield of hydroxyl ((OH)-O-center dot) radicals and degradation of 4-CP under visible light illumination. All results indicated that as-fabricated AgBr/TiO2 NTAs photoelectrode displayed superior PC performance, which was mainly ascribed to the intense visible light absorbance and high charge separation efficiency. Moreover, the intermediates and toxification change during PC degradation of 4-CP were elucidated according to the UPLC-MS/MS measurement and luminescent bacterial tests.
内容类型期刊论文
源URL[http://ir.isl.ac.cn/handle/363002/34440]  
专题青海盐湖研究所_盐湖资源综合利用工程技术中心
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Cui, Yuqi,Zhang, Zixuan,Li, Bo,et al. Ultrasound assisted fabrication of AgBr TiO2 nano-tube arrays photoelectrode and its enhanced visible photocatalytic performance and mechanism for detoxification of 4-chlorphenol[J]. SEPARATION AND PURIFICATION TECHNOLOGY,2018,197:189-196.
APA Cui, Yuqi.,Zhang, Zixuan.,Li, Bo.,Guo, Ruonan.,Zhang, Xinyi.,...&Cheng, Qingfeng.(2018).Ultrasound assisted fabrication of AgBr TiO2 nano-tube arrays photoelectrode and its enhanced visible photocatalytic performance and mechanism for detoxification of 4-chlorphenol.SEPARATION AND PURIFICATION TECHNOLOGY,197,189-196.
MLA Cui, Yuqi,et al."Ultrasound assisted fabrication of AgBr TiO2 nano-tube arrays photoelectrode and its enhanced visible photocatalytic performance and mechanism for detoxification of 4-chlorphenol".SEPARATION AND PURIFICATION TECHNOLOGY 197(2018):189-196.
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