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Recycling waste plastics packaging to value-added products by two-step microwave cracking with different heating strategies
Jing, Xiaodong1,3; Wen, Hao1; Gong, Xuzhong2,3; Xu, Zhihong1; Kajetanowicz, Anna4
刊名FUEL PROCESSING TECHNOLOGY
2020-05-01
卷号201页码:17
关键词Microwave cracking Heating strategy Spherical activated carbon Columnar activated carbon Two-step method
ISSN号0378-3820
DOI10.1016/j.fuproc.2020.106346
英文摘要Waste plastics packaging (WPP) was converted into valuable products by two-step microwave cracking. The wax (38.47-72.53 wt%), gas (20.18-43.85 wt%) and solid (2.00-24.18 wt%) were produced in the first step, and the liquid (60.55-79.94 wt%), gas (18.44-38.45 wt%) and solid (1.00-5.56 wt%) were produced in the second step. Different heating strategies including the selection of absorbers and catalyst, the adjustment of heating power, the mass ratio of absorber to feedstock have been proposed to optimize the products in each step. Commercial spherical activated carbon, columnar activated carbon and molecular sieves type 4A have been used as absorbers and catalysts. The gas products (mainly H-2, CH4, C2H4 and C3H6) can be used as combustion gas. The solid products (mainly CaO, TiO2 and SiO2) in the first step are suitable for absorbers because of their fast temperature rise (30-115 degrees C/min) in microwave field. The liquid products are distributed between C-7 and C-25, which are suitable for gasoline and diesel fractions. Absorbers have been used many times to reduce costs. Two-step method can effectively remove plastic additives, and other attachments in the first step, and the separation of 'dirty' process and 'clean' process can reduce the possibility of catalyst deactivation due to impurity coverage.
资助项目National Natural Science Foundation of China[21776288/U1610101] ; National R&D Infrastructure and Facility Development Program of China ; Fundamental Science Data Sharing Platform[DKA2017-12-02-05] ; CAS informatization project during the Thirteenth Five-Year Plan "Key Database Construction and Application Services for the Discipline of Chemistry"[XXH1350303-103]
WOS关键词CATALYTIC PYROLYSIS ; ASSISTED PYROLYSIS ; POLYPROPYLENE ; POLYETHYLENE ; VALORIZATION ; GASOLINE ; HDPE
WOS研究方向Chemistry ; Energy & Fuels ; Engineering
语种英语
出版者ELSEVIER
WOS记录号WOS:000521519800015
资助机构National Natural Science Foundation of China ; National R&D Infrastructure and Facility Development Program of China ; Fundamental Science Data Sharing Platform ; CAS informatization project during the Thirteenth Five-Year Plan "Key Database Construction and Application Services for the Discipline of Chemistry"
内容类型期刊论文
源URL[http://ir.ipe.ac.cn/handle/122111/39889]  
专题中国科学院过程工程研究所
通讯作者Jing, Xiaodong
作者单位1.Chinese Acad Sci, State Key Lab Multiphase Complex Syst, Beijing Engn Res Ctr Proc Pollut Control, Inst Proc Engn, 1,2nd North St, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Natl Engn Lab Hydromet Cleaner Prod Technol, Inst Proc Engn, 1,2nd North St, Beijing 100190, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Univ Warsaw Zwirki & Wigury, Organometall Synth Lab, Biol & Chem Res Ctr, Fac Chem, PL-10102089 Warsaw, Poland
推荐引用方式
GB/T 7714
Jing, Xiaodong,Wen, Hao,Gong, Xuzhong,et al. Recycling waste plastics packaging to value-added products by two-step microwave cracking with different heating strategies[J]. FUEL PROCESSING TECHNOLOGY,2020,201:17.
APA Jing, Xiaodong,Wen, Hao,Gong, Xuzhong,Xu, Zhihong,&Kajetanowicz, Anna.(2020).Recycling waste plastics packaging to value-added products by two-step microwave cracking with different heating strategies.FUEL PROCESSING TECHNOLOGY,201,17.
MLA Jing, Xiaodong,et al."Recycling waste plastics packaging to value-added products by two-step microwave cracking with different heating strategies".FUEL PROCESSING TECHNOLOGY 201(2020):17.
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