Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible-Light CO2 Reduction with a SnS2/SnO2 Junction

doi:10.1002/ange.201912069

	Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible-Light CO2 Reduction with a SnS2/SnO2 Junction
	You, Feifei 1,2; Wan, Jiawei 1; Qi, Jian 1,2; Mao, Dan 1,2; Yang, Nailiang 1,2; Zhang, Qinghua 3; Gu, Lin 3; Wang, Dan 1,2
刊名	ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
	2020-01-07
卷号	59 期号:2 页码:721-724
关键词	CO2 photoreduction hollow structures lattice distortion multi-shells tin
ISSN号	1433-7851
DOI	10.1002/ange.201912069
英文摘要	Precise control of the micro-/nanostructures of nanomaterials, such as hollow multi-shelled structures (HoMSs), has shown its great advantages in various applications. Now, the crystal structure of building blocks of HoMSs are controlled by introducing the lattice distortion in HoMSs, for the first time. The lattice distortion located at the nanoscale interface of SnS2/SnO2 can provide additional active sites, which not only provide the catalytic activity under visible light but also improve the separation of photoexcited electron-hole pairs. Combined with the efficient light utilization, the natural advantage of HoMSs, a record catalytic activity was achieved in solid-gas system for CO2 reduction, with an excellent stability and 100% CO selectivity without using any sensitizers or noble metals.
资助项目	National Natural Science Foundation of China[21590795] ; National Natural Science Foundation of China[21821005] ; National Natural Science Foundation of China[51772296] ; National Natural Science Foundation of China[51772294] ; National Natural Science Foundation of China[51702321] ; National Natural Science Foundation of China[51972306] ; National Natural Science Foundation of China[51802306] ; National Key R&D Program of China[2016YFB0600903] ; Youth Innovation Promotion Association of CAS[2017070]
WOS关键词	MICROSPHERES ; PHOTOCATALYSTS ; PERFORMANCE
WOS研究方向	Chemistry
语种	英语
出版者	WILEY-V C H VERLAG GMBH
WOS记录号	WOS:000505279500029
资助机构	National Natural Science Foundation of China ; National Key R&D Program of China ; Youth Innovation Promotion Association of CAS
内容类型	期刊论文
源URL	[http://ir.ipe.ac.cn/handle/122111/39204]
专题	中国科学院过程工程研究所
通讯作者	Wang, Dan
作者单位	1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 North 2nd St, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 10049, Peoples R China 3.Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China
推荐引用方式 GB/T 7714	You, Feifei,Wan, Jiawei,Qi, Jian,et al. Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible-Light CO2 Reduction with a SnS2/SnO2 Junction[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2020,59(2):721-724.
APA	You, Feifei.,Wan, Jiawei.,Qi, Jian.,Mao, Dan.,Yang, Nailiang.,...&Wang, Dan.(2020).Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible-Light CO2 Reduction with a SnS2/SnO2 Junction.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,59(2),721-724.
MLA	You, Feifei,et al."Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible-Light CO2 Reduction with a SnS2/SnO2 Junction".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 59.2(2020):721-724.