Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible Light CO2 Reduction with a SnS2/SnO2 Junction | |
You, Feifei1,2; Wan, Jiawei1; Qi, Jian1,2; Mao, Dan1,2; Yang, Nailiang1,2; Zhang, Qinghua3; Gu, Lin3; Wang, Dan1,2 | |
刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION |
2019-11-13 | |
页码 | 5 |
关键词 | CO2 photoreduction hollow structures lattice distortion multi-shells tin |
ISSN号 | 1433-7851 |
DOI | 10.1002/anie.201912069 |
英文摘要 | Precise control of the micro-/nanostructures of nanomaterials, such as hollow multi-shelled structures (HoMSs), has shown its great advantages in various applications. Now, the crystal structure of building blocks of HoMSs are controlled by introducing the lattice distortion in HoMSs, for the first time. The lattice distortion located at the nanoscale interface of SnS2/SnO2 can provide additional active sites, which not only provide the catalytic activity under visible light but also improve the separation of photoexcited electron-hole pairs. Combined with the efficient light utilization, the natural advantage of HoMSs, a record catalytic activity was achieved in solid-gas system for CO2 reduction, with an excellent stability and 100 % CO selectivity without using any sensitizers or noble metals. |
资助项目 | National Natural Science Foundation of China[21590795] ; National Natural Science Foundation of China[21821005] ; National Natural Science Foundation of China[51772296] ; National Natural Science Foundation of China[51772294] ; National Natural Science Foundation of China[51702321] ; National Natural Science Foundation of China[51972306] ; National Natural Science Foundation of China[51802306] ; National Key R&D Program of China[2016YFB0600903] ; Youth Innovation Promotion Association of CAS[2017070] |
WOS关键词 | MICROSPHERES ; PHOTOCATALYSTS ; PERFORMANCE |
WOS研究方向 | Chemistry |
语种 | 英语 |
出版者 | WILEY-V C H VERLAG GMBH |
WOS记录号 | WOS:000496012300001 |
资助机构 | National Natural Science Foundation of China ; National Key R&D Program of China ; Youth Innovation Promotion Association of CAS |
内容类型 | 期刊论文 |
源URL | [http://ir.ipe.ac.cn/handle/122111/39037] |
专题 | 中国科学院过程工程研究所 |
通讯作者 | Wang, Dan |
作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 North 2nd St, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 10049, Peoples R China 3.Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China |
推荐引用方式 GB/T 7714 | You, Feifei,Wan, Jiawei,Qi, Jian,et al. Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible Light CO2 Reduction with a SnS2/SnO2 Junction[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2019:5. |
APA | You, Feifei.,Wan, Jiawei.,Qi, Jian.,Mao, Dan.,Yang, Nailiang.,...&Wang, Dan.(2019).Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible Light CO2 Reduction with a SnS2/SnO2 Junction.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,5. |
MLA | You, Feifei,et al."Lattice Distortion in Hollow Multi-Shelled Structures for Efficient Visible Light CO2 Reduction with a SnS2/SnO2 Junction".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019):5. |
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