Residues of organochlorine pesticides (OCPs) and polycyclic aromatic hydrocarbons (PAHs) in waters of the Ili-Balkhash Basin, arid Central Asia: Concentrations and risk assessment

	Residues of organochlorine pesticides (OCPs) and polycyclic aromatic hydrocarbons (PAHs) in waters of the Ili-Balkhash Basin, arid Central Asia: Concentrations and risk assessment
	Shen, Beibei; Wu, Jinglu; Zhan, Shuie; Jin, Miao
刊名	CHEMOSPHERE
	2021
卷号	273
英文摘要	Release and transport of contaminants in watersheds can have adverse effects on aquatic organisms and human health. Little attention, however, has been paid to chemical contamination of aquatic environments in arid regions by persistent organic pollutants. We analyzed the concentrations and distributions of organochlorine pesticides (OCPs) and polycyclic aromatic hydrocarbons (PAHs) in waters of the Ili-Balkhash Basin, in arid central Asia. Sigma OCP concentrations ranged from 4.02 to 122.80 ng L-1 and Sigma PAH concentrations were between 7.58 and 70.98 ng L-1. On a global scale, OCP and PAH concentrations in waters of the Ili-Balkhash system were relatively low, with only a few exceptions, i.e., highest concentrations near cities and relatively high values in some headwater areas. Source identification revealed that the dichlorodiphenyltrichloroethanes (DDTs) may come from recent use, whereas endosulfans stem from historic applications. Lindane, a common insecticide, may be responsible for hexachlorocyclohexanes (HCHs). Low-molecular-weight PAHs, primarily originating from wood and coal combustion and petroleum-derived sources, were the primary components of PAHs in waters. Furthermore, the primary sources of PAHs at different sites were identified using a Positive Matrix Factorization model: 1) oil leakage (33.9%), 2) biomass burning (29.5%), 3) coal combustion (22.6%), and 4) petroleum-powered vehicles (14.1%). Agricultural, industrial and domestic activities are all potential pollution sources. Besides, contaminated headwater areas indicate that long-range transport has probably become a non-negligible mechanism for pollutant distribution. Risk assessment showed low to moderate toxicity for aquatic organisms, but no marked carcinogenic or non-carcinogenic risks for human health. (C) 2021 Elsevier Ltd. All rights reserved.
内容类型	期刊论文
源URL	[http://159.226.73.51/handle/332005/20522]
专题	中国科学院南京地理与湖泊研究所
推荐引用方式 GB/T 7714	Shen, Beibei,Wu, Jinglu,Zhan, Shuie,et al. Residues of organochlorine pesticides (OCPs) and polycyclic aromatic hydrocarbons (PAHs) in waters of the Ili-Balkhash Basin, arid Central Asia: Concentrations and risk assessment[J]. CHEMOSPHERE,2021,273.
APA	Shen, Beibei,Wu, Jinglu,Zhan, Shuie,&Jin, Miao.(2021).Residues of organochlorine pesticides (OCPs) and polycyclic aromatic hydrocarbons (PAHs) in waters of the Ili-Balkhash Basin, arid Central Asia: Concentrations and risk assessment.CHEMOSPHERE,273.
MLA	Shen, Beibei,et al."Residues of organochlorine pesticides (OCPs) and polycyclic aromatic hydrocarbons (PAHs) in waters of the Ili-Balkhash Basin, arid Central Asia: Concentrations and risk assessment".CHEMOSPHERE 273(2021).