Chemical source profiles of particulate matter and gases emitted from solid fuels for residential cooking and heating scenarios in Qinghai-Tibetan Plateau

doi:10.1016/j.envpol.2021.117503

CORC > 地球环境研究所 > 中国科学院地球环境研究所 > 粉尘与环境研究室

	Chemical source profiles of particulate matter and gases emitted from solid fuels for residential cooking and heating scenarios in Qinghai-Tibetan Plateau
	Sun, Jian 1,2; Shen, Zhenxing 1,2; Zhang, Bin 1; Zhang, Leiming 3; Zhang, Yue 1; Zhang, Qian 4; Wang, Diwei 1; Huang, Yu 2; Liu, Suixin 2; Cao, Junji 2
刊名	ENVIRONMENTAL POLLUTION
	2021-09-15
卷号	285 页码:10
关键词	Dung cake combustion Emission factor PAHs VOCs Pollutants source profiles
ISSN号	0269-7491
DOI	10.1016/j.envpol.2021.117503
通讯作者	Shen, Zhenxing(zxshen@mail.xjtu.edu.cn)
英文摘要	Incomplete combustion of solid fuels (animal dung and bituminous coal) is a common phenomenon during residential cooking and heating in the Qinghai-Tibetan Plateau (QTP), resulting in large amounts of pollutants emitted into the atmosphere. This study investigated the pollutant emissions from six burning scenarios (heating and cooking with each of the three different fuels: yak dung, sheep dung, and bitumite) in the QTP's pastoral dwellings. Target pollutants such as carbon monoxide (CO), gas-phase polycyclic aromatic hydrocarbons (PAHs), volatile organic compounds (VOCs), fine particles (PM2.5, particulate matter with an aerodynamic diameter < 2.5 mu m), carbonaceous aerosols, water-soluble ions, and particle-phase PAHs were investigated. Emission factors (EFs) (mean +/- standard deviation) of PM2.5 from the six scenarios were in the range of 1.21 +/- 0.47-7.03 +/- 1.95 g kg(-1), of which over 60% mass fractions were carbonaceous aerosols. The ratio of organic carbon to elemental carbon ranged from 9.6 +/- 2.7-33.4 +/- 11.5 and 81.7 +/- 30.4-91.9 +/- 29.0 for dung and bitumite burning, respectively. These values were much larger than those reported in the literature, likely because of the region's high altitudes-where the oxygen level is approximately 65% of that at the sea level-thus providing a deficient air supply to stoves. However, the toxicity and carcinogenicity of PAHs emitted from solid fuel combustion in the QTP are significant, despite a slightly lower benzo(a)pyrene-equivalent carcinogenic potency (Bap(eq)) in this study than in the literature. The gas-to-particle partitioning coefficient of PAHs and VOC emission profiles in the QTP differed significantly from those reported for other regions in the literature. More attention should be paid to the emissions of PAH derivatives (oxygenated PAHs and nitro-PAHs), considering their enhanced lightabsorbing ability and high BaPeq from solid fuel combustion in the QTP.
资助项目	National Natural Science Foundation of China[41877383] ; National Natural Science Foundation of China[41907188] ; Hunan Provincial Key Research and Development Program[2018SK2039] ; SKLLQG, Chinese Academy of Sciences[SKLLQG1919] ; China Postdoctoral Science Foundation[2019M653658]
WOS关键词	POLYCYCLIC AROMATIC-HYDROCARBONS ; ORGANIC-COMPOUNDS VOCS ; EMISSION FACTORS ; COAL COMBUSTION ; HOUSEHOLD STOVES ; GUANZHONG PLAIN ; AIR-POLLUTION ; YAK DUNG ; CARBONACEOUS PARTICLES ; SEASONAL-VARIATION
WOS研究方向	Environmental Sciences & Ecology
语种	英语
出版者	ELSEVIER SCI LTD
WOS记录号	WOS:000685348400001
资助机构	National Natural Science Foundation of China ; Hunan Provincial Key Research and Development Program ; SKLLQG, Chinese Academy of Sciences ; China Postdoctoral Science Foundation
内容类型	期刊论文
源URL	[http://ir.ieecas.cn/handle/361006/16924]
专题	地球环境研究所_粉尘与环境研究室
通讯作者	Shen, Zhenxing
作者单位	1.Xi An Jiao Tong Univ, Dept Environm Sci & Engn, Xian 710049, Peoples R China 2.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710049, Peoples R China 3.Environm & Climate Change Canada, Sci & Technol Branch, Air Qual Res Div, Toronto, ON, Canada 4.Xian Univ Architecture & Technol, Key Lab Northwest Resource Environm & Ecol, MOE, Xian 710055, Peoples R China
推荐引用方式 GB/T 7714	Sun, Jian,Shen, Zhenxing,Zhang, Bin,et al. Chemical source profiles of particulate matter and gases emitted from solid fuels for residential cooking and heating scenarios in Qinghai-Tibetan Plateau[J]. ENVIRONMENTAL POLLUTION,2021,285:10.
APA	Sun, Jian.,Shen, Zhenxing.,Zhang, Bin.,Zhang, Leiming.,Zhang, Yue.,...&Cao, Junji.(2021).Chemical source profiles of particulate matter and gases emitted from solid fuels for residential cooking and heating scenarios in Qinghai-Tibetan Plateau.ENVIRONMENTAL POLLUTION,285,10.
MLA	Sun, Jian,et al."Chemical source profiles of particulate matter and gases emitted from solid fuels for residential cooking and heating scenarios in Qinghai-Tibetan Plateau".ENVIRONMENTAL POLLUTION 285(2021):10.