Radiation effect on ionic liquid [Hbet][Tf2N] for Nd(2)O(3)separation from simulated spent nuclear fuels | |
Fan, Fang-Li1; Chen, De-Sheng1,3; Huang, Qing-Gang1; Wang, Jie-Ru1,2,3; Tan, Cun-Min1; Wu, Xiao-Lei1; Qin, Zhi1,3 | |
刊名 | JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY |
2020-08-02 | |
页码 | 6 |
关键词 | Ionic liquid Radiation stability Spent nuclear fuel Dissolution separation |
ISSN号 | 0236-5731 |
DOI | 10.1007/s10967-020-07306-2 |
通讯作者 | Fan, Fang-Li(fanfangli@impcas.ac.cn) ; Qin, Zhi(qinzhi@impcas.ac.cn) |
英文摘要 | Radiation-chemical stability of ionic liquid [Hbet][Tf2N] has been investigated under gamma irradiation for Nd(2)O(3)separation from simulated spent nuclear fuels. It was found that Nd(2)O(3)dissolution decreases with increasing absorbed dose of [Hbet][Tf2N]. However, the dissolution ability of irradiated [Hbet][Tf2N] to Nd(2)O(3)can be regenerated after washing with water. The radiolytic products of [Hbet][Tf2N] were identified by EMI-MS, and [Hbet](+)group occurred a little radiolysis during irradiation. The UV-Visible spectra shown an increase in absorption around 275 nm probably due to the radiolysis of [Hbet][Tf2N]. FTIR spectra shown little variation around 1730 cm(-1)under high radiation dose. |
资助项目 | Strategic Priority Research Program of Chinese Academy of Sciences[XDA21010202] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDA03010402] ; Young Scholar of CAS Light of West China Program[2016-84] ; Natural Sciences Foundation of Gansu Province[17JR5RA298] |
WOS关键词 | RARE-EARTH-ELEMENTS ; BAUXITE RESIDUE ; STABILITY ; EXTRACTION ; CHEMISTRY ; GAMMA ; SEPARATIONS ; LANTHANIDE ; CATIONS ; SYSTEM |
WOS研究方向 | Chemistry ; Nuclear Science & Technology |
语种 | 英语 |
出版者 | SPRINGER |
WOS记录号 | WOS:000554849000001 |
资助机构 | Strategic Priority Research Program of Chinese Academy of Sciences ; Young Scholar of CAS Light of West China Program ; Natural Sciences Foundation of Gansu Province |
内容类型 | 期刊论文 |
源URL | [http://119.78.100.186/handle/113462/140203] |
专题 | 中国科学院近代物理研究所 |
通讯作者 | Fan, Fang-Li; Qin, Zhi |
作者单位 | 1.Chinese Acad Sci, Inst Modern Phys, Lanzhou, Peoples R China 2.Lanzhou Univ, Sch Nucl Sci & Technol, Lanzhou, Peoples R China 3.Univ Chinese Acad Sci, Sch Nucl Sci & Technol, Beijing, Peoples R China |
推荐引用方式 GB/T 7714 | Fan, Fang-Li,Chen, De-Sheng,Huang, Qing-Gang,et al. Radiation effect on ionic liquid [Hbet][Tf2N] for Nd(2)O(3)separation from simulated spent nuclear fuels[J]. JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY,2020:6. |
APA | Fan, Fang-Li.,Chen, De-Sheng.,Huang, Qing-Gang.,Wang, Jie-Ru.,Tan, Cun-Min.,...&Qin, Zhi.(2020).Radiation effect on ionic liquid [Hbet][Tf2N] for Nd(2)O(3)separation from simulated spent nuclear fuels.JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY,6. |
MLA | Fan, Fang-Li,et al."Radiation effect on ionic liquid [Hbet][Tf2N] for Nd(2)O(3)separation from simulated spent nuclear fuels".JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY (2020):6. |
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