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Mo-doped SnO2 nanotubes sensor with abundant oxygen vacancies for ethanol detection
Wang, Li1; Ma, Shuyi1; Li, Jianpeng2,3; Wu, Andong2; Luo, Didi2; Yang, Tingting1; Cao, Pengfei1; Ma, Nina1; Cai, Yahui1
刊名SENSORS AND ACTUATORS B-CHEMICAL
2021-11-15
卷号347页码:11
关键词Oxygen vacancy Mo doping SnO2 Gas sensor Electrostatic spinning
DOI10.1016/j.snb.2021.130642
通讯作者Ma, Shuyi(wangli5787@163.com)
英文摘要This work describes a synthesizing method for Mo-doped SnO2 nanotubes (NTs) with uniform morphology by combining electrostatic spinning and air sintering. The method uses Mo ions to do substitutional doping of Sn ions in SnO2 to construct new lattice defects (such as oxygen vacancies), which provides more active sites for gas adsorption. Ethanol was taken as an example to study gas sensitivity characteristics of synthesized products. The analysis showed that 5 mol% of Mo-doped SnO2 nanotubes sensor exhibited the highest response (46.8) to 100 ppm ethanol at a lower optimum temperature (220 degrees C) and reduced the response/recovery time to 7/103 s. Also, it manifested excellent selectivity and long-term stability. The functionalized nanotubes structure and optimized parameters (oxygen vacancies concentration, metal vacancies defects, carrier concentration, catalytic sites, and base resistance increased) are the reasons for enhancing gas-sensing performance. This work provides direction that the optimal doping concentration of transition metal elements for metal-oxide NTs gas sensors can achieve the best sensing response.
资助项目National Natural Science Foundation of China[11864034] ; National Natural Science Foundation of China[11964035] ; key research project of the Chinese Academy of Sciences[QYZDY-SSW-JSC019]
WOS关键词GAS SENSOR ; ROOM-TEMPERATURE ; SENSING PERFORMANCE ; ZNO ; HYDROGEN ; NANOPARTICLES ; FILM ; HETEROJUNCTIONS ; NANOFIBERS ; DESIGN
WOS研究方向Chemistry ; Electrochemistry ; Instruments & Instrumentation
语种英语
出版者ELSEVIER SCIENCE SA
WOS记录号WOS:000697559500004
资助机构National Natural Science Foundation of China ; key research project of the Chinese Academy of Sciences
内容类型期刊论文
源URL[http://119.78.100.186/handle/113462/136521]  
专题中国科学院近代物理研究所
通讯作者Ma, Shuyi
作者单位1.Northwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R China
2.Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Peoples R China
3.Lanzhou Univ, Sch Phys Sci & Technol, 222 South Tianshui Rd, Lanzhou 730000, Peoples R China
推荐引用方式
GB/T 7714
Wang, Li,Ma, Shuyi,Li, Jianpeng,et al. Mo-doped SnO2 nanotubes sensor with abundant oxygen vacancies for ethanol detection[J]. SENSORS AND ACTUATORS B-CHEMICAL,2021,347:11.
APA Wang, Li.,Ma, Shuyi.,Li, Jianpeng.,Wu, Andong.,Luo, Didi.,...&Cai, Yahui.(2021).Mo-doped SnO2 nanotubes sensor with abundant oxygen vacancies for ethanol detection.SENSORS AND ACTUATORS B-CHEMICAL,347,11.
MLA Wang, Li,et al."Mo-doped SnO2 nanotubes sensor with abundant oxygen vacancies for ethanol detection".SENSORS AND ACTUATORS B-CHEMICAL 347(2021):11.
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