Electrochemical-Osmotic Process for Simultaneous Recovery of Electric Energy, Water, and Metals from Wastewater
Sun, Meng; Qin, Mohan; Wang, Chi; Weng, Guoming; Huo, Mingxin; Taylor, Andre D.; Qu, Jiuhui; Elimelech, Menachem
刊名ENVIRONMENTAL SCIENCE & TECHNOLOGY
2020-07-07
卷号54期号:13页码:8430-8442
ISSN号0013-936X
英文摘要A highly-efficient, autonomous electrochemical-osmotic system (EOS) is developed for simultaneous recovery of electric energy, water, and metals from wastewater. We demonstrate that the system can generate a maximum electric power density of 10.5 W m(-2) using a spontaneous Fe/Cu2+ galvanic cell, while simultaneously achieving copper recovery from wastewater. With an osmotic pressure difference generated by the deployed electrochemical reactions, water is osmotically extracted from the feed solution with the EOS at a water flux of 5.1 L m(-2) h(-1). A scaled-up EOS realizes a power density of 105.8 W per m(-3) of treated water to light an LED over 24 h while also enhancing water extraction and metal recovery. The modularized EOS obtains ultrahigh (>97.5%) Faradaic efficiencies under variable operating conditions, showing excellent system stability. The EOS is also versatile: it can recover Au, Ag, and Hg from wastewaters with simultaneous electricity and water coproduction. Our study demonstrates a promising pathway for realizing multi-resource recycling from wastewater by coupling electrochemical and osmosis-driven processes.
内容类型期刊论文
源URL[http://ir.rcees.ac.cn/handle/311016/45282]  
专题生态环境研究中心_中国科学院饮用水科学与技术重点实验室
推荐引用方式
GB/T 7714
Sun, Meng,Qin, Mohan,Wang, Chi,et al. Electrochemical-Osmotic Process for Simultaneous Recovery of Electric Energy, Water, and Metals from Wastewater[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2020,54(13):8430-8442.
APA Sun, Meng.,Qin, Mohan.,Wang, Chi.,Weng, Guoming.,Huo, Mingxin.,...&Elimelech, Menachem.(2020).Electrochemical-Osmotic Process for Simultaneous Recovery of Electric Energy, Water, and Metals from Wastewater.ENVIRONMENTAL SCIENCE & TECHNOLOGY,54(13),8430-8442.
MLA Sun, Meng,et al."Electrochemical-Osmotic Process for Simultaneous Recovery of Electric Energy, Water, and Metals from Wastewater".ENVIRONMENTAL SCIENCE & TECHNOLOGY 54.13(2020):8430-8442.
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