Decabromodiphenyl Ether versus Decabromodiphenyl Ethane: Source, Fate, and Influencing Factors in a Coastal Sea Nearing Source Region

doi:10.1021/acs.est.0c08528

CORC > 烟台海岸带研究所 > 中国科学院烟台海岸带研究所 > 中科院海岸带环境过程与生态修复重点实验室 > 近岸生态与环境实验室

	Decabromodiphenyl Ether versus Decabromodiphenyl Ethane: Source, Fate, and Influencing Factors in a Coastal Sea Nearing Source Region
	Zhen, Xiaomei 1,2,3,4; Li, Yanfang 2,3,4; Tang, Jianhui 2,3,6; Wang, Xinming 1; Liu, Lin 2,3,4; Zhong, Mingyu 5; Tian, Chongguo 2,3,6
刊名	ENVIRONMENTAL SCIENCE & TECHNOLOGY
	2021-06-01
卷号	55 期号:11 页码:7376-7385
关键词	brominated flame retardants source and sink multi-box mass balance model river discharge atmospheric deposition BDE 209/DBDPE ratio Bohai Sea
ISSN号	0013-936X
DOI	10.1021/acs.est.0c08528
通讯作者	Tang, Jianhui(jhtang@yic.ac.cn)
英文摘要	Both decabromodiphenyl ether (BDE 209) and decabromodiphenyl ethane (DBDPE) are still produced in large quantities in China, especially in the Shandong Province closed to the Bohai Sea (BS). This study conducted a comprehensive investigation of the distribution and budget of brominated flame retardants (BFRs) in the BS. BDE 209 was the predominant BFR in most of the investigated rivers flowing into the BS, although DBDPE exceeded BDE 209 in certain rivers as a result of the replacement of BDE 209 with DBDPE in North China. The spatial distributions of BFRs in the rivers were controlled by the proximity of the BFR manufacturing base and the extent of urbanization. BFRs' spatial distribution in the BS was influenced by a combination of land-based pollution sources, environmental parameters (e.g., suspended particulate matter, particulate organic carbon, and particulate black carbon), and hydrodynamic conditions. The spatial variation trend of BDE 209/DBDPE ratios in various environmental media provided useful information. Vertically, the BDE 209/DBDPE ratio decreased from the seawater surface layer to the sediment, indicating their differential transport in the BS. A multi-box mass balance model and analysis of BDE 209 showed that degradation was the primary sink of BFRs in seawater (similar to 68%) and surface sediment (similar to 72%) in the BS.
资助项目	National Natural Science Foundation of China (NSFC) ; Shandong Province Joint Fund[U1806207] ; NSFC[41773138] ; key project of Chinese Academy of Sciences[XDA11020402] ; key deployment project of Centre for Ocean Mega-Science, Chinese Academy of Sciences[COMS2019J08] ; seed project of Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences[YIC Y855011024]
WOS关键词	POLYBROMINATED DIPHENYL ETHERS ; HALOGENATED FLAME RETARDANTS ; LONG-RANGE TRANSPORT ; BOHAI SEA ; DECHLORANE PLUS ; SPATIAL-DISTRIBUTION ; YELLOW SEA ; SEASONAL-VARIATION ; SURFACE SEDIMENTS ; RIVER DELTA
WOS研究方向	Engineering ; Environmental Sciences & Ecology
语种	英语
WOS记录号	WOS:000659374200019
资助机构	National Natural Science Foundation of China (NSFC) ; Shandong Province Joint Fund ; NSFC ; key project of Chinese Academy of Sciences ; key deployment project of Centre for Ocean Mega-Science, Chinese Academy of Sciences ; seed project of Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences
内容类型	期刊论文
源URL	[http://ir.yic.ac.cn/handle/133337/29424]
专题	烟台海岸带研究所_近岸生态与环境实验室烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
通讯作者	Tang, Jianhui
作者单位	1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510631, Peoples R China 2.Chinese Acad Sci, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res YIC, Yantai 264003, Peoples R China 3.YICCAS, Shandong Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China 4.Univ Chinese Acad Sci UCAS, Beijing 100049, Peoples R China 5.Yantai Univ, Yantai 264005, Shandong, Peoples R China 6.Chinese Acad Sci, Ctr Ocean Megasci, Qingdao 266071, Peoples R China
推荐引用方式 GB/T 7714	Zhen, Xiaomei,Li, Yanfang,Tang, Jianhui,et al. Decabromodiphenyl Ether versus Decabromodiphenyl Ethane: Source, Fate, and Influencing Factors in a Coastal Sea Nearing Source Region[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2021,55(11):7376-7385.
APA	Zhen, Xiaomei.,Li, Yanfang.,Tang, Jianhui.,Wang, Xinming.,Liu, Lin.,...&Tian, Chongguo.(2021).Decabromodiphenyl Ether versus Decabromodiphenyl Ethane: Source, Fate, and Influencing Factors in a Coastal Sea Nearing Source Region.ENVIRONMENTAL SCIENCE & TECHNOLOGY,55(11),7376-7385.
MLA	Zhen, Xiaomei,et al."Decabromodiphenyl Ether versus Decabromodiphenyl Ethane: Source, Fate, and Influencing Factors in a Coastal Sea Nearing Source Region".ENVIRONMENTAL SCIENCE & TECHNOLOGY 55.11(2021):7376-7385.