Influence of carbon nano-dots in water on sonoluminescence | |
Song, Dan2,3; Xu, Wen2,4,5; Luo, Man1; Zhang, Mingjun1; Wen, Hua2,3; Cheng, Xingjia2,3; Luo, Xiaobing1; Wang, Zhibiao1 | |
刊名 | NANOSCALE |
2021-06-29 | |
ISSN号 | 2040-3364 |
DOI | 10.1039/d1nr02194j |
通讯作者 | Xu, Wen(wenxu_issp@aliyun.com) ; Wang, Zhibiao(wangzb@cqmu.edu.cn) |
英文摘要 | Sonoluminescence (SL) occurs when acoustically induced oscillating bubbles in a liquid collapse. The SL from pure water normally generates ultraviolet to blue emission which is related to hydroxyl plasma formed in and around the bubbles. It is known that carbon nano-dots (CNDs) can serve as free radical captors, where the C-bonds can couple strongly with free radicals and form C-based functional groups. In this work, a SL experiment is conducted via placing CND aqueous solution (CNDAS) in the focal area of the SL apparatus. Unexpectedly and dramatically, it is found that the color of SL now turns orange, which is so bright that it can be seen even by the naked eye. By examining the CNDAS before and after the SL experiment, it is observed that the influence of CNDs on optical absorption, photoluminescence and SL is mainly achieved via coupling between the C-bonds in the CNDs and the free hydroxyl radicals generated during the processes of acoustically driven cavitation and SL. The interesting and important findings from this work demonstrate that the CNDs in water can modify significantly the SL effect. Thus, CNDs can provide a new test medium for studying and revealing the microscopic mechanism of the SL phenomenon. |
资助项目 | National Natural Science foundation of China[U206720039] ; National Natural Science foundation of China[U193010069] ; National Science foundation of China[81127901] |
WOS关键词 | GRAPHENE QUANTUM DOTS ; SINGLE-BUBBLE ; ULTRASOUND ; EMISSION ; IONS ; RECOMBINATION ; FLUORESCENCE ; CAVITATION ; EFFICIENCY ; RADICALS |
WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
语种 | 英语 |
出版者 | ROYAL SOC CHEMISTRY |
WOS记录号 | WOS:000683438300001 |
资助机构 | National Natural Science foundation of China ; National Science foundation of China |
内容类型 | 期刊论文 |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/124315] |
专题 | 中国科学院合肥物质科学研究院 |
通讯作者 | Xu, Wen; Wang, Zhibiao |
作者单位 | 1.Chongqing Med Univ, Coll Biomed Engn, Key Lab Ultrasound Med & Engn, Chongqing 400010, Peoples R China 2.Chinese Acad Sci, Inst Solid State Phys, HFIPS, Key Lab Mat Phys, Hefei 230031, Peoples R China 3.Univ Sci & Technol China, Hefei 230026, Peoples R China 4.Yunnan Univ, Yunnan Key Lab Quantum Informat, Kunming 650000, Yunnan, Peoples R China 5.Yunnan Univ, Sch Phys & Astron, Kunming 650000, Yunnan, Peoples R China |
推荐引用方式 GB/T 7714 | Song, Dan,Xu, Wen,Luo, Man,et al. Influence of carbon nano-dots in water on sonoluminescence[J]. NANOSCALE,2021. |
APA | Song, Dan.,Xu, Wen.,Luo, Man.,Zhang, Mingjun.,Wen, Hua.,...&Wang, Zhibiao.(2021).Influence of carbon nano-dots in water on sonoluminescence.NANOSCALE. |
MLA | Song, Dan,et al."Influence of carbon nano-dots in water on sonoluminescence".NANOSCALE (2021). |
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