Interfacial Approach toward Benzene-Bridged Polypyrrole Film-Based Micro-Supercapacitors with Ultrahigh Volumetric Power Density | |
Jiang, KY; Baburin, IA; Han, P; Yang, CQ; Fu, XB; Yao, YF; Li, JT; Canovas, E; Seifert, G; Chen, JS | |
刊名 | ADVANCED FUNCTIONAL MATERIALS |
2019 | |
页码 | - |
关键词 | HIGH-PERFORMANCE CONDUCTING POLYPYRROLE ORGANIC FRAMEWORKS MONOLAYER CAPACITOR ANALOGS |
ISSN号 | 1616-301X |
DOI | 10.1002/adfm.201908243 |
文献子类 | 期刊论文 |
英文摘要 | 2D soft nanomaterials are an emerging research field due to their versatile chemical structures, easily tunable properties, and broad application potential. In this study, a benzene-bridged polypyrrole film with a large area, up to a few square centimeters, is synthesized through an interfacial polymerization approach. As-prepared semiconductive films exhibit a bandgap of approximate to 2 eV and a carrier mobility of approximate to 1.5 cm(2) V-1 s(-1), inferred from time-resolved terahertz spectroscopy. The samples are employed to fabricate in-plane micro-supercapacitors (MSCs) by laser scribing and exhibit an ultrahigh areal capacitance of 0.95 mF cm(-2), using 1-ethyl-3-methylimidazolium tetrafluoroborate ([EMIM][BF4]) as an electrolyte. Importantly, the maximum energy and power densities of the developed MSCs reach values up to 50.7 mWh cm(-3) and 9.6 kW cm(-3), respectively; the performance surpassing most of the 2D material-based MSCs is reported to date. |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.sinap.ac.cn/handle/331007/32104] |
专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
作者单位 | 1.East China Normal Univ, Shanghai Key Lab Magnet Resonance, North Zhongshan Rd 3663, Shanghai 200062, Peoples R China; 2.Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai Key Lab Elect Insulat & Thermal Ageing, State Key Lab Met Matrix Composites,Soft2D Lab, Shanghai 200240, Peoples R China; 3.Tech Univ Dresden, Ctr Advancing Elect Dresden, D-01062 Dresden, Germany; 4.Tech Univ Dresden, Dept Chem & Food Chem, D-01062 Dresden, Germany; 5.Max Planck Inst Polymer Res, Ackermannweg 10, D-55128 Mainz, Germany; 6.East China Normal Univ, Phys Dept, North Zhongshan Rd 3663, Shanghai 200062, Peoples R China; 7.Chinese Acad Sci, Shanghai Inst Appl Phys, Dept Molten Salt Chem & Engn, Shanghai 201800, Peoples R China; 8.KTH Royal Inst Technol, Sch Informat & Commun Technol, Electrum 229, S-16440 Kista, Sweden; 9.Inst Madrileno Estudios Avanzados Nanociencia IMD, Faraday 9, Madrid 28049, Spain; 10.Changzhou Univ, Sch Mat Sci & Engn, Jiangsu Key Lab Environmentally Friendly Polymer, Changzhou 213164, Peoples R China |
推荐引用方式 GB/T 7714 | Jiang, KY,Baburin, IA,Han, P,et al. Interfacial Approach toward Benzene-Bridged Polypyrrole Film-Based Micro-Supercapacitors with Ultrahigh Volumetric Power Density[J]. ADVANCED FUNCTIONAL MATERIALS,2019:-. |
APA | Jiang, KY.,Baburin, IA.,Han, P.,Yang, CQ.,Fu, XB.,...&Zhuang, XD.(2019).Interfacial Approach toward Benzene-Bridged Polypyrrole Film-Based Micro-Supercapacitors with Ultrahigh Volumetric Power Density.ADVANCED FUNCTIONAL MATERIALS,-. |
MLA | Jiang, KY,et al."Interfacial Approach toward Benzene-Bridged Polypyrrole Film-Based Micro-Supercapacitors with Ultrahigh Volumetric Power Density".ADVANCED FUNCTIONAL MATERIALS (2019):-. |
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