A reaction-based ratiometric fluorescent probe for mercury ion detection in aqueous solution
Liu, Shudi1; Feng, Di2; Zhang, Liangwei3; Song, He1; Wang, Yue3; Zhang, Xia3; Zhao, Qingjun1; Chen, Lingxin3
刊名SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY
2020-12-15
卷号243页码:6
关键词Fluorescent probe Mercury ion Detection Ratiometric Fluorescence imaging
ISSN号1386-1425
DOI10.1016/j.saa.2020.118817
通讯作者Zhang, Liangwei(liangweizhang@yic.ac.cn) ; Chen, Lingxin(lxchen@yic.ac.cn)
英文摘要Mercury ions are crucially harmful to ecosystem and human being due to their characters of bioaccumulation and difficulty of biochemical degradation. Therefore, development of mercury ion detection methods has attracted increasing interests recently. In this study, we successfully synthesized a hydroxyphenylbenzothiazole (HBT)based fluorescent probe HBT-Hg in an extremely simple manner for mercuric ions detection. The spectral studies revealed that the probe HBT-Hg could react with Hg2+ selectively and sensitively in PBS buffer (10 mM, pH = 7.40), showing ratiometric fluorescent changes from blue to light green. The response mechanism of the probe HBT-Hg and Hg2+ was finally confirmed by HPLC analysis, viz., the probe HBT-Hg converted to its precursor compound 1. Finally, the probe HBT-Hg was successfully applied in monitoring Hg2+ in living A549 cells. (c) 2020 Elsevier B.V. All rights reserved.
资助项目Natural Science Foundation of China[21701074] ; Natural Science Foundation of China[21778026] ; Natural Science Foundation of China[21976209] ; Natural Science Foundation of China[21402077] ; program of Youth Innovation Pro-motion Association, CAS[2019217] ; Taishan Scholar Project Special Funding[TS20190962]
WOS关键词HG2+ ; FLUORIDE ; CHEMOSENSORS ; BOND
WOS研究方向Spectroscopy
语种英语
WOS记录号WOS:000576843300002
资助机构Natural Science Foundation of China ; program of Youth Innovation Pro-motion Association, CAS ; Taishan Scholar Project Special Funding
内容类型期刊论文
源URL[http://ir.yic.ac.cn/handle/133337/28425]  
专题烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
烟台海岸带研究所_山东省海岸带环境工程技术研究中心
通讯作者Zhang, Liangwei; Chen, Lingxin
作者单位1.Yantai Univ, Coll Chem & Chem Engn, Yantai 264005, Peoples R China
2.Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Qingdao 266042, Peoples R China
3.Chinese Acad Sci, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Res Ctr Coastal Environm Engn & Technol, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China
推荐引用方式
GB/T 7714
Liu, Shudi,Feng, Di,Zhang, Liangwei,et al. A reaction-based ratiometric fluorescent probe for mercury ion detection in aqueous solution[J]. SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY,2020,243:6.
APA Liu, Shudi.,Feng, Di.,Zhang, Liangwei.,Song, He.,Wang, Yue.,...&Chen, Lingxin.(2020).A reaction-based ratiometric fluorescent probe for mercury ion detection in aqueous solution.SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY,243,6.
MLA Liu, Shudi,et al."A reaction-based ratiometric fluorescent probe for mercury ion detection in aqueous solution".SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY 243(2020):6.
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