Preparation of mixed-matrix membranes from metal organic framework (MIL-53) and poly (vinylidene fluoride) for use in determination of sulfonylurea herbicides in aqueous environments by high performance liquid chromatography
Ma, JP; Li, S; Wu, GG; Wang, SS; Guo, XT; Wang, LY; Wang, XY; Li, JH; Chen, LX
刊名JOURNAL OF COLLOID AND INTERFACE SCIENCE
2019-10-01
卷号553页码:834-844
关键词Sulfonylurea herbicides (SUs) Dispersion membrane extraction (DME) Metal-organic frameworks (MOFs) Mixed-matrix membrane (MMM) Aqueous environments
ISSN号0021-9797
DOI10.1016/j.jcis.2019.06.082
产权排序[Ma, Jiping ; Li, Shuang ; Wu, Gege ; Wang, Shasha] Qingdao Univ Technol, State Local Joint Engn Res Ctr Urban Sewage Treat, Sch Environm & Municipal Engn, Qingdao 266033, Shandong, Peoples R China ; [Guo, Xiaotong ; Wang, Liyan ; Wang, Xiaoyan ; Li, Jinhua ; Chen, Lingxin] Chinese Acad Sci, Yantai Inst Coastal Zone Res, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China ; [Guo, Xiaotong ; Wang, Liyan ; Wang, Xiaoyan ; Li, Jinhua ; Chen, Lingxin] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Res Ctr Coastal Environm Engn & Technol, Yantai 264003, Peoples R China ; [Guo, Xiaotong ; Wang, Liyan] Univ Chinese Acad Sci, Beijing 100049, Peoples R China ; [Chen, Lingxin] Qufu Normal Univ, Coll Chem & Chem Engn, Qufu 273165, Peoples R China
文献子类Article
英文摘要Novel mixed-matrix membranes (MMM) were prepared from metal-organic frameworks (MOF) (MIL-53) and poly (vinylidene fluoride) (PVDF), viz MIL-53-PVDF MMM, for the simultaneous dispersion membrane extraction (DME) of seven sulfonylurea herbicides (SUs) in aqueous environments followed by high performance liquid chromatography (HPLC) determination. The MIL-53-PVDF MMM was well characterized and major factors influencing DME performances were systematically investigated including membrane type, MOF dosage, eluent type, solution pH, extraction/elution time and salinity, etc. Under optimal conditions, the MIL-53-PVDF MMM based DME coupled with HPLC exhibited excellent linearity within 0.03-10 mu g L-1 for chlorimuronethyl and 0.01-10 mu g L-1 for other six SUs individual. High enrichment factor of 250 was obtained, as well as low detection limits and quantification limits ranged from 3.75 to 10.30 ng L-1 and 12.49-34.30 ng L-1, respectively. Furthermore, the method attained high recoveries of 77.20-111.00% at three spiking levels of SUs, with relative standard deviations of 1.28-14.67% in tap water, seawater and surface water samples. Additionally, the MMM was readily separated from water and well regenerated, and could keep about 80% recovery after 25 cycles. Compared to that reported extraction materials, the MIL-53-PVDF MMM possessed the advantages of high enrichment ability, excellent reusability, good practicality and easy separation, indicating it was a promising alternative for the enrichment of SUs from aqueous environments. (C) 2019 Elsevier Inc. All rights reserved.
WOS关键词SOLID-PHASE EXTRACTION ; POLYCYCLIC AROMATIC-HYDROCARBONS ; WATER SAMPLES ; TRACE ANALYSIS ; ULTRAFILTRATION MEMBRANES ; THIFENSULFURON-METHYL ; CARBON NANOTUBES ; RECENT PROGRESS ; F-MOFS ; EFFICIENT
WOS研究方向Chemistry, Physical
语种英语
WOS记录号WOS:000483454400087
资助机构National Natural Science Foundation of ChinaNational Natural Science Foundation of China [21547002, 21804010, 21876199] ; Natural Science Foundation of Shandong ProvinceNatural Science Foundation of Shandong Province [ZR2019MB046] ; Department of Science and Technology of Shandong Province of China [GG201709290055]
内容类型期刊论文
源URL[http://ir.yic.ac.cn/handle/133337/24851]  
专题烟台海岸带研究所_山东省海岸带环境工程技术研究中心
烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
作者单位1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China;
2.Qufu Normal Univ, Coll Chem & Chem Engn, Qufu 273165, Peoples R China
3.Qingdao Univ Technol, State Local Joint Engn Res Ctr Urban Sewage Treat, Sch Environm & Municipal Engn, Qingdao 266033, Shandong, Peoples R China;
4.Chinese Acad Sci, Yantai Inst Coastal Zone Res, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China;
5.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Res Ctr Coastal Environm Engn & Technol, Yantai 264003, Peoples R China;
推荐引用方式
GB/T 7714
Ma, JP,Li, S,Wu, GG,et al. Preparation of mixed-matrix membranes from metal organic framework (MIL-53) and poly (vinylidene fluoride) for use in determination of sulfonylurea herbicides in aqueous environments by high performance liquid chromatography[J]. JOURNAL OF COLLOID AND INTERFACE SCIENCE,2019,553:834-844.
APA Ma, JP.,Li, S.,Wu, GG.,Wang, SS.,Guo, XT.,...&Chen, LX.(2019).Preparation of mixed-matrix membranes from metal organic framework (MIL-53) and poly (vinylidene fluoride) for use in determination of sulfonylurea herbicides in aqueous environments by high performance liquid chromatography.JOURNAL OF COLLOID AND INTERFACE SCIENCE,553,834-844.
MLA Ma, JP,et al."Preparation of mixed-matrix membranes from metal organic framework (MIL-53) and poly (vinylidene fluoride) for use in determination of sulfonylurea herbicides in aqueous environments by high performance liquid chromatography".JOURNAL OF COLLOID AND INTERFACE SCIENCE 553(2019):834-844.
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