Activating microwave absorption performance by reduced graphene oxide-borophene heterostructure
Wang, Shipeng1,2; Li, Qingsong1,2; Hu, Kang1,2; Liu, Qiangchun1,2; Liu, Xiaofang4; Kong, Xiangkai1,2,3
刊名COMPOSITES PART A-APPLIED SCIENCE AND MANUFACTURING
2020-11-01
卷号138
关键词Graphene Borophene Metal-free Microwave absorption
ISSN号1359-835X
DOI10.1016/j.compositesa.2020.106033
通讯作者Liu, Qiangchun(qchliu@chnu.edu.cn) ; Liu, Xiaofang(liuxf05@buaa.edu.cn) ; Kong, Xiangkai(kxk@chnu.edu.cn)
英文摘要Reduced graphene oxide (RGO) nanosheets normally possess large specific surface area, good electrical conductivity, and low density, but their unsatisfactory intrinsic complex permittivity and poor impedance matching severely hinder the further application in microwave adsorption. In this work, borophene nanosheets (BNS), the lightest 2D material, are proposed as an efficient activator to improve the microwave absorbing performance on RGO. BNS are assembled and im-mobilized on RGO surface through the interfacial covalent interaction, to construct a new metal-free 2D hybrid absorbent. These incorporated BNS serves as the joining site and channel in the framework to facilitate electrons hopping and migration between RGO layers. As a result, conducive loss mechanism is well enhanced, which is the major contribution to its dielectric property, conferring high impedance matching on the absorbent. As expected, the as-obtained 2D metal-free hybrid demonstrates microwave absorbing parameters that approach those of the most active absorbents, with the minimum reflection loss reaching -53.3 dB and the broadest effective absorption bandwidth of 6.16 GHz, at a low filler loading of 3 wt %.
资助项目National Nature Science Foundation of China[U1832138] ; National Nature Science Foundation of China[51602116] ; Anhui Provincial Natural Science Foundation[1508085ME100] ; Anhui Provincial Natural Science Foundation[1708085QB40] ; Anhui Provincial Natural Science Fund for Colleges and Universities[KJ2017ZD31] ; China Postdoctoral Science Foundation[2016M600492]
WOS关键词ELECTROMAGNETIC-WAVE ABSORPTION ; NANOCOMPOSITES ; LIGHTWEIGHT ; COMPOSITES ; POLYANILINE ; FABRICATION ; EFFICIENCY ; ABSORBERS ; NANOSHEET
WOS研究方向Engineering ; Materials Science
语种英语
出版者ELSEVIER SCI LTD
WOS记录号WOS:000576639500009
资助机构National Nature Science Foundation of China ; Anhui Provincial Natural Science Foundation ; Anhui Provincial Natural Science Fund for Colleges and Universities ; China Postdoctoral Science Foundation
内容类型期刊论文
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/104440]  
专题中国科学院合肥物质科学研究院
通讯作者Liu, Qiangchun; Liu, Xiaofang; Kong, Xiangkai
作者单位1.Huaibei Normal Univ, Anhui Prov Key Lab Pollutant Sensit Mat & Environ, Huaibei 235000, Anhui, Peoples R China
2.Huaibei Normal Univ, Key Lab Green & Precise Synthet Chem & Applicat, Minist Educ, Huaibei 235000, Anhui, Peoples R China
3.Chinese Acad Sci, High Magnet Field Lab, Hefei 230031, Anhui, Peoples R China
4.Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China
推荐引用方式
GB/T 7714
Wang, Shipeng,Li, Qingsong,Hu, Kang,et al. Activating microwave absorption performance by reduced graphene oxide-borophene heterostructure[J]. COMPOSITES PART A-APPLIED SCIENCE AND MANUFACTURING,2020,138.
APA Wang, Shipeng,Li, Qingsong,Hu, Kang,Liu, Qiangchun,Liu, Xiaofang,&Kong, Xiangkai.(2020).Activating microwave absorption performance by reduced graphene oxide-borophene heterostructure.COMPOSITES PART A-APPLIED SCIENCE AND MANUFACTURING,138.
MLA Wang, Shipeng,et al."Activating microwave absorption performance by reduced graphene oxide-borophene heterostructure".COMPOSITES PART A-APPLIED SCIENCE AND MANUFACTURING 138(2020).
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