A reinvestigation of low molecular weight components in SOA produced by cyclohexene ozonolysis

doi:10.1007/s41365-018-0491-0

CORC > 合肥物质科学研究院 > 中国科学院合肥物质科学研究院 > 中科院安徽光学精密机械研究所

	A reinvestigation of low molecular weight components in SOA produced by cyclohexene ozonolysis
	Chen, Jun 4; Li, Zhao-Hui 4; Yu, Ye-Peng 4; Lin, Xuan 4; Zhang, Hang 4; Li, Yan-Bo 4; Wang, Huan-Huan 4; Sun, Rui-Rui 4; Meng, Qing-Hui 4; Huang, Chao-Qun 3
刊名	NUCLEAR SCIENCE AND TECHNIQUES
	2018-11-01
卷号	29 期号:11 页码:9
关键词	Cyclohexene Ozonolysis SOA Smog chamber Aerosol mass spectrometry
ISSN号	1001-8042
DOI	10.1007/s41365-018-0491-0
通讯作者	Huang, Chao-Qun(cqhuang@aiofm.ac.cn) ; Liu, Fu-Yi(fyliu@ustc.edu.cn)
英文摘要	The ozonolysis of cyclohexene is an important model system for understanding the more complex reaction of O-3 with monoterpenes; however, many previous studies have come to qualitatively different conclusions about the composition of the secondary organic aerosol (SOA) formed in this system. In the present study, the composition of the SOA produced by cyclohexene ozonolysis in the absence of seed aerosols has been investigated online and off-line using synchrotron-based thermal desorption/tunable vacuum ultraviolet photoionization time-of-flight aerosol mass spectrometry (TD-VUV-TOF-PIAMS) in conjunction with a custom-built smog chamber. On the basis of the molecular ions observed by mass spectrometry at 11.5eV, it was found that dicarboxylic acids, dialdehydes, and cyclic anhydrides are the predominant low molecular weight components in the particle phase. The results also indicated that TD-VUV-TOF-PIAMS coupled with filter sampling is a potentially useful tool for the investigation of SOA composition both in the field and in the laboratory.
资助项目	National Natural Science Foundation of China[11575178] ; National Natural Science Foundation of China[91544105] ; National Natural Science Foundation of China[U1532137] ; National Natural Science Foundation of China[91544228] ; National Natural Science Foundation of China[U1232130]
WOS关键词	SECONDARY ORGANIC AEROSOL ; GAS-PHASE ; MASS-SPECTROMETRY ; PHOTOIONIZATION ; PARTICLES ; OXIDATION ; OZONE ; PHOTOOXIDATION ; CHAMBER ; O-3
WOS研究方向	Nuclear Science & Technology ; Physics
语种	英语
出版者	SPRINGER SINGAPORE PTE LTD
WOS记录号	WOS:000446031200002
资助机构	National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China
内容类型	期刊论文
源URL	[http://ir.hfcas.ac.cn:8080/handle/334002/40214]
专题	合肥物质科学研究院_中科院安徽光学精密机械研究所
通讯作者	Huang, Chao-Qun; Liu, Fu-Yi
作者单位	1.Univ Sci & Technol China, Sch Environm Sci & Optoelect Technol, Hefei 230026, Anhui, Peoples R China 2.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Lab Atmospher Physicochem, Hefei 230031, Anhui, Peoples R China 3.Chinese Acad Sci, Hefei Inst Phys Sci, Ctr Med Phys & Technol, Lab Med Opt & Mass Spectrometry, 350 Shushanhu Rd, Hefei 230031, Anhui, Peoples R China 4.Univ Sci & Technol China, Sch Nucl Sci & Technol, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China
推荐引用方式 GB/T 7714	Chen, Jun,Li, Zhao-Hui,Yu, Ye-Peng,et al. A reinvestigation of low molecular weight components in SOA produced by cyclohexene ozonolysis[J]. NUCLEAR SCIENCE AND TECHNIQUES,2018,29(11):9.
APA	Chen, Jun.,Li, Zhao-Hui.,Yu, Ye-Peng.,Lin, Xuan.,Zhang, Hang.,...&Sheng, Liu-Si.(2018).A reinvestigation of low molecular weight components in SOA produced by cyclohexene ozonolysis.NUCLEAR SCIENCE AND TECHNIQUES,29(11),9.
MLA	Chen, Jun,et al."A reinvestigation of low molecular weight components in SOA produced by cyclohexene ozonolysis".NUCLEAR SCIENCE AND TECHNIQUES 29.11(2018):9.