Ultrahigh Surface Area N-Doped Hierarchically Porous Carbon for Enhanced CO2 Capture and Electrochemical Energy Storage

doi:10.1002/cssc.201901137

	Ultrahigh Surface Area N-Doped Hierarchically Porous Carbon for Enhanced CO2 Capture and Electrochemical Energy Storage
	Wang, Shuai 1,2; Qin, Jieqiong 3,4; Zhao, Yujuan 1,2; Duan, Linlin 1,2; Wang, Jinxiu 1,2; Gao, Wenjun 1,2; Wang, Ruicong 1,2; Wang, Changyao 1,2; Pal, Manas 1,2; Wu, Zhong-Shuai 3
刊名	CHEMSUSCHEM
	2019-08-08
卷号	12 期号:15 页码:3541-3549
关键词	CO2 capture hierarchical pore structure nitrogen-doping porous carbon supercapacitor
ISSN号	1864-5631
DOI	10.1002/cssc.201901137
通讯作者	Li, Wei(weilichem@fudan.edu.cn) ; Zhao, Dongyuan(dyzhao@fudan.edu.cn)
英文摘要	Facile synthesis of ultrahigh surface area porous carbons with well-defined functionalities such as N-doping remains a formidable challenge as extensive pore creation results in significant damage to the active sites. Herein, an ultrahigh surface area, N-doped hierarchically porous carbon was prepared through a multicomponent co-assembly approach. The resultant N-doped hierarchically porous carbon (N-HPC) possessed an ultrahigh surface area (approximate to 1960 m(2) g(-1)), a uniform interpenetrating micropore (approximate to 1.3 nm) and large mesopore (approximate to 7.6 nm) size, and high N-doping in the carbon frameworks (approximate to 5 wt %). The N-HPC exhibited a high specific capacitance (358 F g(-1) at 0.5 A g(-1)) as a supercapacitor electrode in aqueous alkaline electrolyte with a stable cycling performance after10 000 charge/discharge cycles. Moreover, as a CO2 absorbent, N-HPC displayed an adsorption capacity of 29.0 mmol g(-1) at 0 degrees C under a high pressure of 30 bar.
WOS关键词	ORDERED MESOPOROUS CARBONS ; WATER-IN-SALT ; NITROGEN-CONTENT ; PERFORMANCE ; FABRICATION ; VOLTAGE ; SUPERCAPACITORS ; CAPACITANCE ; ELECTROLYTE ; BIOCARBONS
WOS研究方向	Chemistry ; Science & Technology - Other Topics
语种	英语
出版者	WILEY-V C H VERLAG GMBH
WOS记录号	WOS:000479276700015
内容类型	期刊论文
源URL	[http://cas-ir.dicp.ac.cn/handle/321008/173195]
专题	大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者	Li, Wei; Zhao, Dongyuan
作者单位	1.Fudan Univ, Adv Mat Lab, Dept Chem, Shanghai Key Lab Mol Catalysis & Innovat Mat iChE, Shanghai 200433, Peoples R China 2.Fudan Univ, State Key Lab Mol Engn Polymers, Shanghai 200433, Peoples R China 3.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, 457 Zhongshan Rd, Dalian 116023, Peoples R China 4.Univ Chinese Acad Sci, 19 A Yuquan Rd, Beijing 100049, Peoples R China
推荐引用方式 GB/T 7714	Wang, Shuai,Qin, Jieqiong,Zhao, Yujuan,et al. Ultrahigh Surface Area N-Doped Hierarchically Porous Carbon for Enhanced CO2 Capture and Electrochemical Energy Storage[J]. CHEMSUSCHEM,2019,12(15):3541-3549.
APA	Wang, Shuai.,Qin, Jieqiong.,Zhao, Yujuan.,Duan, Linlin.,Wang, Jinxiu.,...&Zhao, Dongyuan.(2019).Ultrahigh Surface Area N-Doped Hierarchically Porous Carbon for Enhanced CO2 Capture and Electrochemical Energy Storage.CHEMSUSCHEM,12(15),3541-3549.
MLA	Wang, Shuai,et al."Ultrahigh Surface Area N-Doped Hierarchically Porous Carbon for Enhanced CO2 Capture and Electrochemical Energy Storage".CHEMSUSCHEM 12.15(2019):3541-3549.