Pyrite delta S-34 and Delta S-33 constraints on sulfur cycling at sublacustrine hydrothermal vents in Yellowstone Lake, Wyoming, USA

doi:10.1016/j.gca.2019.09.004

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	Pyrite delta S-34 and Delta S-33 constraints on sulfur cycling at sublacustrine hydrothermal vents in Yellowstone Lake, Wyoming, USA
	Fowler, Andrew P. G.1,6; Liu, Qiu-li 4,5; Huang, Yongshu 4,5; Tan, Chunyang 6; Volk, Michael W. R.3,6; Shanks, W. C. Pat, III 2; Seyfried, William, Jr.6
刊名	GEOCHIMICA ET COSMOCHIMICA ACTA
	2019-11-15
卷号	265 页码:148-162
关键词	Yellowstone Lake SIMS Sulfur isotopes Pyrite Pyrrhotite Sublacustrine Hydrothermal dynamics
ISSN号	0016-7037
DOI	10.1016/j.gca.2019.09.004
英文摘要	Sulfur isotope values (delta S-34 and Delta S-33) of pyrite in sediment from steam-heated hydrothermal vents on the floor of Yellow-stone Lake ( WY) were measured using secondary ionization mass spectrometry (SIMS). The high resolution of the SIMS data place important constraints on sulfur cycling processes at/near the vent fluid-lake water interface. Pyrite with a distinct mantle-basalt (delta S-34 = 0 parts per thousand) isotope composition (delta S-34 = +0.5 to +3.1 parts per thousand) replaces pyrrhotite during incipient stages of alteration at moderately high temperature. Disseminated cubic pyrite (delta S-34 = +2.0 to +5.3 parts per thousand) occurs in zones where more extensive oxidation is likely. Framboidal pyrite with delta S-34 values ranging from -5.2 to +4.1 parts per thousand and Delta S-33 up to +0.30 parts per thousand suggest formation from low-temperature microbial sulfate reduction in sediments near but not directly in the vent fluid up-flow zone. The co-occurrence of pyrite with S isotope values characteristic of distinct formation processes, coupled with notable intracrystal S isotope variations, suggests the venting locus is dynamic in time and space. (C) 2019 Elsevier Ltd. All rights reserved.
资助项目	National Key R&D Program of China[2016YFE0203000] ; NSF[EAR 1515377] ; NSF[OCE 1434798] ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota
WOS关键词	AQUEOUS SULFIDE SOLUTIONS ; SULFATE REDUCTION ; SEDIMENTARY PYRITE ; ISOTOPE FRACTIONATION ; CHIMNEY MINERALS ; HYDROGEN-SULFIDE ; POLYSULFIDE IONS ; S-33 CONSTRAINTS ; STABLE-ISOTOPE ; DEGREES-C
WOS研究方向	Geochemistry & Geophysics
语种	英语
出版者	PERGAMON-ELSEVIER SCIENCE LTD
WOS记录号	WOS:000488959900010
资助机构	National Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota ; National Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota ; National Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota ; National Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota
内容类型	期刊论文
源URL	[http://ir.iggcas.ac.cn/handle/132A11/93928]
专题	地质与地球物理研究所_岩石圈演化国家重点实验室
通讯作者	Fowler, Andrew P. G.
作者单位	1.EHS Support, Pittsburgh, PA 15237 USA 2.US Geol Survey, Denver Fed Ctr, MS 973, Denver, CO 80225 USA 3.Harvard Univ, Dept Earth & Planetary Sci, 20 Oxford St, Cambridge, MA 02138 USA 4.Univ Chinese Acad Sci, Coll Earth Sci, Beijing 100049, Peoples R China 5.Chinese Acad Sci, Inst Geol & Geophys, State Key Lab Lithospher Evolut, Beijing 100029, Peoples R China 6.Univ Minnesota, Dept Earth Sci, Minneapolis, MN 55455 USA
推荐引用方式 GB/T 7714	Fowler, Andrew P. G.,Liu, Qiu-li,Huang, Yongshu,et al. Pyrite delta S-34 and Delta S-33 constraints on sulfur cycling at sublacustrine hydrothermal vents in Yellowstone Lake, Wyoming, USA[J]. GEOCHIMICA ET COSMOCHIMICA ACTA,2019,265:148-162.
APA	Fowler, Andrew P. G..,Liu, Qiu-li.,Huang, Yongshu.,Tan, Chunyang.,Volk, Michael W. R..,...&Seyfried, William, Jr..(2019).Pyrite delta S-34 and Delta S-33 constraints on sulfur cycling at sublacustrine hydrothermal vents in Yellowstone Lake, Wyoming, USA.GEOCHIMICA ET COSMOCHIMICA ACTA,265,148-162.
MLA	Fowler, Andrew P. G.,et al."Pyrite delta S-34 and Delta S-33 constraints on sulfur cycling at sublacustrine hydrothermal vents in Yellowstone Lake, Wyoming, USA".GEOCHIMICA ET COSMOCHIMICA ACTA 265(2019):148-162.