Photocatalytic treatment of 2,4,6-trinitotoluene in red water by multi-doped TiO2 with enhanced visible light photocatalytic activity | |
Zhang, Yihe ; Cheng, Keke ; Lv, Fengzhu ; Huang, Hongwei ; Fei, Bin ; He, Ying ; Ye, Zhengfang ; Shen, Bo | |
刊名 | colloids and surfaces a physicochemical and engineering aspects
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2014 | |
关键词 | Red water Multi-doped TiO2 Photocatalytic Visible light TITANIUM-DIOXIDE DEGRADATION SURFACE NANOTUBES POWDERS |
DOI | 10.1016/j.colsurfa.2014.03.086 |
英文摘要 | Fe-N-doped TiO2, Fe-S-doped TiO2 and Fe-N-S-doped TiO2 were prepared with Fe doping peroxotitanium complex (Fe-PTC) as precursor in aqueous solution by a low-temperature process. The structure and properties of catalysts were characterized by XRD, FT-IR, XPS, TEM and UV-Vis respectively. Fe-N-doped TiO2, Fe-S-doped TiO2 and Fe-N-S-doped TiO2 all belong to anatase phase. The UV-Vis spectra of doped TiO2 exhibited a red shift to 535 nm and stronger absorption than that of pure TiO2 in visible region. The pure TiO2 displays bullet-like morphology with widths of about 20 nm and Fe-N-S-doped TiO2 consisted of irregular particles with diameters about 5-10 nm. The doped samples all exhibited higher photocatalytic activity in the degradation of 2,4,6-trinitotoluene (TNT) in red water compared to pure TiO2. Fe-N-S-doped TiO2 presented the highest photocatalytic activity and degraded about 91.5% 2,4,6-trinitotoluene within 12 h under visible light irradiation. Structural characterization and property analysis results revealed that the co-doping of Fe-N, Fe-S and Fe-N-S remarkably altered the crystal specific surface area, microstructure, as well as the photocatalytic activity. (C) 2014 Elsevier B.V. All rights reserved.; Chemistry, Physical; SCI(E); EI; 5; ARTICLE; zyh@cugb.edu.cn; 1; 103-108; 452 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/212197] ![]() |
专题 | 环境科学与工程学院 |
推荐引用方式 GB/T 7714 | Zhang, Yihe,Cheng, Keke,Lv, Fengzhu,et al. Photocatalytic treatment of 2,4,6-trinitotoluene in red water by multi-doped TiO2 with enhanced visible light photocatalytic activity[J]. colloids and surfaces a physicochemical and engineering aspects,2014. |
APA | Zhang, Yihe.,Cheng, Keke.,Lv, Fengzhu.,Huang, Hongwei.,Fei, Bin.,...&Shen, Bo.(2014).Photocatalytic treatment of 2,4,6-trinitotoluene in red water by multi-doped TiO2 with enhanced visible light photocatalytic activity.colloids and surfaces a physicochemical and engineering aspects. |
MLA | Zhang, Yihe,et al."Photocatalytic treatment of 2,4,6-trinitotoluene in red water by multi-doped TiO2 with enhanced visible light photocatalytic activity".colloids and surfaces a physicochemical and engineering aspects (2014). |
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