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Low-cost nanocarbon electrodes on arbitrary fibrous substrates as efficient bifacial photovoltaic wires
Liu, Wen ; Peng, Ming ; Chen, Si ; Zou, Dechun ; Zhang, Chaoqun ; Fang, Yueping ; Cai, Xin
刊名RSC ADVANCES
2017
关键词SENSITIZED SOLAR-CELLS FLEXIBLE ENERGY-STORAGE COUNTER ELECTRODES CARBON-FIBERS CONVERSION EFFICIENCY HIGHLY EFFICIENT HIGH-PERFORMANCE SOLID-STATE PEN INK DEVICES
DOI10.1039/c6ra27211h
英文摘要The emergence of wearable electronics has demanded advances in efficient flexible/wearable energy devices. Photovoltaic wires (PVWs) have unique 3D light-harvesting capabilities and available electrode materials that are attractive for this purpose. Developing low-cost and efficient Pt-free fibrous counter electrodes (CEs) for PVWs is essential. Herein, ultralow-cost nanocarbon, with considerable electrochemical activity, was deposited onto arbitrary fibers, including TiO2 semiconductor, metal wires, and polymeric carbon fibers, using a facile dip-coating method. These fibers were then used as efficient catalytic fibrous CEs in PVWs. The influence of nanocarbon loading and charge transfer resistance on electrocatalytic activity were investigated in nanocarbon-penetrated Ti/TiO2 nanotube array CEs and dummy cells based on SS wire/nanocarbon CEs. Due to the balanced influences of conductive substrate and nanocarbon electrocatalytic film, PVWs assembled from SS wire/nanocarbon CE and an all-carbon carbon fiber/nanocarbon CE achieved efficiencies of 6.09% and 5.10% under AM1.5G illumination (100 mW cm(-2)), respectively. Furthermore, a double-sided illuminated PVW had an apparent efficiency of 10.8%. This work demonstrates innovative cost-efficient photovoltaic wires that may help boost low-cost, bifacial and highly flexible/wearable photovoltaics toward practical applications.; Natural Science Foundation of China [NSFC 51602109, NSFC 91333107]; Guangdong Provincial Science and Technology Project [2016A050502048, 2014A030310427]; SCI(E); ARTICLE; 16; 9653-9661; 7
语种英语
内容类型期刊论文
源URL[http://ir.pku.edu.cn/handle/20.500.11897/476389]  
专题化学与分子工程学院
推荐引用方式
GB/T 7714
Liu, Wen,Peng, Ming,Chen, Si,et al. Low-cost nanocarbon electrodes on arbitrary fibrous substrates as efficient bifacial photovoltaic wires[J]. RSC ADVANCES,2017.
APA Liu, Wen.,Peng, Ming.,Chen, Si.,Zou, Dechun.,Zhang, Chaoqun.,...&Cai, Xin.(2017).Low-cost nanocarbon electrodes on arbitrary fibrous substrates as efficient bifacial photovoltaic wires.RSC ADVANCES.
MLA Liu, Wen,et al."Low-cost nanocarbon electrodes on arbitrary fibrous substrates as efficient bifacial photovoltaic wires".RSC ADVANCES (2017).
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