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Preparation and photocatalytic performance of titania nanotubes loaded with Ag nanoparticles
Li Hai-Long1; Luo Wu-Lin1; Chen Tao1; Tian Wen-Yu1; Sun Mao1; Li Chun1; Zhu Di1; Liu Ran-Ran1; Zhao Yu-Liang2,3; Liu Chun-Li1
刊名ACTA PHYSICO-CHIMICA SINICA
2008-08-01
卷号24期号:8页码:1383-1386
关键词Nanotubes Titania Ag Hydrothennal Method Photocatalysis
ISSN号1000-6818
DOI10.3866/PKU.WHXB20080810
英文摘要Titania nanotubes (TNTs) were synthesized by hydrothermal treatment of rutile-phase TiO2 nanoparticles in 10 mol center dot L-1 NaOH solution at 110 degrees C for 24 h. The Ag loaded titania nanotubes (Ag/TNTs) were obtained by chemical deposition method with the TNTs suspending in the AgNO3 solution (pH=8) at 50 degrees C. The characterizations of the assynthesized samples were performed by TEM, EDS, XRD, XPS, and UV-Vis spectra. The photocatalytic performance of the Ag/TNTs was investigated by UV-light induced photocatalytic decomposition of methyl orange(MO). The results showed that the inner/outer diameters of TNTs were about 6/10 nm and the length was several hundred nanometers. Both the shape and the crystalline of the nanotubes were not changed after the modification. The zero oxidation state Ag quantum dots, about 4 nm in diameter, were well dispersed on the external surface of the nanotubes. Ag/TNTs exhibited enhanced absorption at the visible range in the UV-Vis spectra. The Ag nanoparticles were found to significantly enhance the photocatalytic activity of TiO2 nanotubes, and the catalyst system was demonstrated to be highly efficient for the UV-light induced photocatalytic decomposition of MO compared to both rutile-phase TiO2 nanoparticles and pure TNTs. After irradiation for 60 min, the decomposition rates of MO solution in rutile-phase TiO2 nanoparticles, TNTs, and Ag/TNTs system were 46.8%, 57.2%, and 92.2%, respectively.
语种英语
出版者PEKING UNIV PRESS
WOS记录号WOS:000259171000010
内容类型期刊论文
源URL[http://ir.iccas.ac.cn/handle/121111/63671]  
专题中国科学院化学研究所
通讯作者Liu Chun-Li
作者单位1.Peking Univ, Beijing Natl Lab Mol Sci, Coll Chem & Mol Engn, Beijing 100871, Peoples R China
2.Chinese Acad Sci, Lab Bioenvironm Hlth Sci Nanoscale Mat & Nanosafe, Inst High Energy Phys, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Key Lab Nucl Analyt Tech, Inst High Energy Phys, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Li Hai-Long,Luo Wu-Lin,Chen Tao,et al. Preparation and photocatalytic performance of titania nanotubes loaded with Ag nanoparticles[J]. ACTA PHYSICO-CHIMICA SINICA,2008,24(8):1383-1386.
APA Li Hai-Long.,Luo Wu-Lin.,Chen Tao.,Tian Wen-Yu.,Sun Mao.,...&Liu Chun-Li.(2008).Preparation and photocatalytic performance of titania nanotubes loaded with Ag nanoparticles.ACTA PHYSICO-CHIMICA SINICA,24(8),1383-1386.
MLA Li Hai-Long,et al."Preparation and photocatalytic performance of titania nanotubes loaded with Ag nanoparticles".ACTA PHYSICO-CHIMICA SINICA 24.8(2008):1383-1386.
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