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Comprehensive studies of response characteristics of organic photodetectors based on rubrene and C-60
Yang, Dezhi; Xu, Kai; Zhou, Xiaokang; Wang, Yanping; Ma, Dongge
刊名JOURNAL OF APPLIED PHYSICS
2014-06-28
卷号115期号:24
ISSN号0021-8979
DOI10.1063/1.4885078
英文摘要We studied the transient response characteristics of organic photodetectors composing of high mobility materials of rubrene and C-60, respectively, as donor and acceptor. It was found that the response speed was limited by the delay time of both exciton diffusion and transit, and an anomalous phenomenon that the bandwidth decreases as the reverse bias increases was found for the first time. The investigation of frequency dependence at different device structures and light excitations demonstrated that the light absorption of rubrene prevents the photodetector from obtaining a fast response. With the help of magnetic field effect study, it was clearly elucidated that the slow diffusion time of the long lifetime triplet excitons generated from singlet fission in rubrene limited the bandwidth of the device. Moreover, the simulation of the response of photodetector under transient and steady state by exciton transport-diffusion equation showed that the exciton dissociation efficiency in rubrene increases more quickly than that in C-60, which should account for the negative dependence of bandwidth on the reverse bias in rubrene-based device. (C) 2014 AIP Publishing LLC.
语种英语
出版者AMER INST PHYSICS
WOS记录号WOS:000338633600051
内容类型期刊论文
源URL[http://ir.iccas.ac.cn/handle/121111/52797]  
专题中国科学院化学研究所
通讯作者Ma, Dongge
作者单位Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Polymer Phys & Chem, Changchun 130022, Peoples R China
推荐引用方式
GB/T 7714
Yang, Dezhi,Xu, Kai,Zhou, Xiaokang,et al. Comprehensive studies of response characteristics of organic photodetectors based on rubrene and C-60[J]. JOURNAL OF APPLIED PHYSICS,2014,115(24).
APA Yang, Dezhi,Xu, Kai,Zhou, Xiaokang,Wang, Yanping,&Ma, Dongge.(2014).Comprehensive studies of response characteristics of organic photodetectors based on rubrene and C-60.JOURNAL OF APPLIED PHYSICS,115(24).
MLA Yang, Dezhi,et al."Comprehensive studies of response characteristics of organic photodetectors based on rubrene and C-60".JOURNAL OF APPLIED PHYSICS 115.24(2014).
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