Ta2O5 Nanowires: a novel synthetic method and their solar energy utilization | |
Lu, Xujie3,4; Ding, Shangjun3,4; Lin, Tianquan3,4; Mou, Xinliang3; Hong, Zhanglian1,2; Huang, Fuqiang3,5,6 | |
刊名 | DALTON TRANSACTIONS
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2012 | |
卷号 | 41期号:2页码:622-627 |
ISSN号 | 1477-9226 |
DOI | 10.1039/c1dt11124h |
英文摘要 | Single-crystalline uniform Ta2O5 nanowires are prepared by a novel synthetic route. The formation of the nanowires involves an oriented attachment process caused by the reduction of surface energy. The nanowires are successfully applied to photocatalytic H-2 evolution, contaminant degradation, and dye-sensitized solar cells (DSCs). The Ta2O5-based DSCs reveal a significant photovoltaic response, which has not been reported. As a photocatalyst, the Ta2O5 nanowires possess high H-2 evolution efficiency under Xe lamp irradiation, nearly 27-fold higher than the commercial powders. A better performance of photocatalytic contaminant degradation is also observed. Such improvements are ascribed to better charge transport ability for the single-crystalline wire and a higher potential energy of the conduction band. This new synthetic approach using a water-soluble precursor provides a versatile way to prepare nanostructured metal oxides. |
语种 | 英语 |
出版者 | ROYAL SOC CHEMISTRY |
WOS记录号 | WOS:000298000000040 |
内容类型 | 期刊论文 |
源URL | [http://ir.iccas.ac.cn/handle/121111/48509] ![]() |
专题 | 中国科学院化学研究所 |
通讯作者 | Hong, Zhanglian |
作者单位 | 1.Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China 2.Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Peoples R China 3.Chinese Acad Sci, Shanghai Inst Ceram, CAS Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China 4.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China 5.Peking Univ, Coll Chem & Mol Engn, Beijing Natl Lab Mol Sci, Beijing 100871, Peoples R China 6.Peking Univ, Coll Chem & Mol Engn, State Key Lab Rare Earth Mat Chem & Applicat, Beijing 100871, Peoples R China |
推荐引用方式 GB/T 7714 | Lu, Xujie,Ding, Shangjun,Lin, Tianquan,et al. Ta2O5 Nanowires: a novel synthetic method and their solar energy utilization[J]. DALTON TRANSACTIONS,2012,41(2):622-627. |
APA | Lu, Xujie,Ding, Shangjun,Lin, Tianquan,Mou, Xinliang,Hong, Zhanglian,&Huang, Fuqiang.(2012).Ta2O5 Nanowires: a novel synthetic method and their solar energy utilization.DALTON TRANSACTIONS,41(2),622-627. |
MLA | Lu, Xujie,et al."Ta2O5 Nanowires: a novel synthetic method and their solar energy utilization".DALTON TRANSACTIONS 41.2(2012):622-627. |
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