Ellipticity-dependent of multiple ionisation methyl iodide cluster using 532 nm nanosecond laser
Tang, Bin1; Zhao, Wuduo2; Wang, Weiguo2; Hua, Lei2; Chen, Ping2; Hou, Keyong2; Huang, Yunguang1; Li, Haiyang2
刊名MOLECULAR PHYSICS
2016-03-18
卷号114期号:6页码:855-861
关键词Multiply Charged Ions Nanosecond Laser Methyl Iodide Cluster Laser Polarisation
ISSN号0026-8976
DOI10.1080/00268976.2015.1127442
文献子类Article
英文摘要The dependence of multiply charged ions on laser ellipticity in methyl iodide clusters with 532nm nanosecond laser was measured using a time-of-flight mass spectrometer. The intensities of multiply charged ions I-q(+)(q = 2-4) with circularly polarised laser pulse were clearly higher than those with linearly polarised laser pulse but the intensity of single charged ions I+ was inverse. And the dependences of ions on the optical polarisation state were investigated and a flower petal and square distribution for single charged ions (I+, C+) and multiply charged ions (I2+, I3+, I4+, C2+) were observed, respectively. A theoretical calculation was also proposed to simulate the distributions of ions and theoretical results fitted well with the experimental ones. It indicated that the high multiphoton ionisation probability in the initial stage would result in the disintegration of big clusters into small ones and suppress the production of multiply charged ions.
WOS关键词MULTIELECTRON DISSOCIATIVE IONIZATION ; ELECTRON-ENERGY DISTRIBUTION ; COULOMB EXPLOSION ; WAVELENGTH DEPENDENCE ; ASSISTANT GENERATION ; ATOMIC CLUSTERS ; IONS ; PULSES ; CH3I ; INTENSITY
WOS研究方向Physics
语种英语
出版者TAYLOR & FRANCIS LTD
WOS记录号WOS:000372129500012
内容类型期刊论文
源URL[http://cas-ir.dicp.ac.cn/handle/321008/170648]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Wang, Weiguo
作者单位1.Guangxi Grid Elect Power Res Inst, Nanning, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Key Lab Separat Sci Analyt Chem, Dalian, Peoples R China
推荐引用方式
GB/T 7714
Tang, Bin,Zhao, Wuduo,Wang, Weiguo,et al. Ellipticity-dependent of multiple ionisation methyl iodide cluster using 532 nm nanosecond laser[J]. MOLECULAR PHYSICS,2016,114(6):855-861.
APA Tang, Bin.,Zhao, Wuduo.,Wang, Weiguo.,Hua, Lei.,Chen, Ping.,...&Li, Haiyang.(2016).Ellipticity-dependent of multiple ionisation methyl iodide cluster using 532 nm nanosecond laser.MOLECULAR PHYSICS,114(6),855-861.
MLA Tang, Bin,et al."Ellipticity-dependent of multiple ionisation methyl iodide cluster using 532 nm nanosecond laser".MOLECULAR PHYSICS 114.6(2016):855-861.
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