Modulating the Electronic Properties of Monolayer Graphene Using a Periodic Quasi-One-Dimensional Potential Generated by Hex-Reconstructed Au(001)
Zhou, Xiebo2,3; Qi, Yue3; Shi, Jianping2,3; Niu, Jingjing1,4; Liu, Mengxi3; Zhang, Guanhua5; Li, Qiucheng3; Zhang, Zhepeng3; Hong, Min2,3; Ji, Qingqing3
刊名ACS NANO
2016-08-01
卷号10期号:8页码:7550-7557
关键词Graphene Scanning Tunneling Microscopy/spectroscopy Atomic Structure New Dirac Points Au(001)
ISSN号1936-0851
DOI10.1021/acsnano.6b02548
文献子类Article
英文摘要The structural and electronic properties of monolayer graphene synthesized on a periodically reconstructed substrate can be widely modulated by the generation of superstructure patterns, thereby producing interesting physical properties, such as magnetism and superconductivity. Herein, using a facile chemical vapor deposition method, we successfully synthesized high-quality monolayer graphene with a uniform thickness on Au foils. The hex-reconstruction of Au(001), which is characterized by striped patterns with a periodicity of 1.44 nm, promoted the formation of a quasi-one-dimensional (1D) graphene superlattice, which served as a periodic quasi-1D modulator for the graphene overlayer, as evidenced by scanning tunneling microscopy/spectroscopy. Intriguingly, two new Dirac points were generated for the quasi-1D graphene superlattice located at -1.73 +/- 0.02 and 1.12 +/- 0.12 eV. Briefly, this work demonstrates that the periodic modulation effect of reconstructed metal substrates can dramatically alter the electronic properties of graphene and provides insight into the modulation of these properties using 1D potentials.
WOS关键词CHEMICAL-VAPOR-DEPOSITION ; HEXAGONAL BORON-NITRIDE ; EPITAXIAL GRAPHENE ; DIRAC FERMIONS ; LARGE-AREA ; POLYCRYSTALLINE GRAPHENE ; GRAIN-BOUNDARIES ; GROWTH ; FILMS ; LAYER
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000381959100037
内容类型期刊论文
源URL[http://cas-ir.dicp.ac.cn/handle/321008/170306]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Wu, Xiaosong; Zhang, Yanfeng
作者单位1.Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China
2.Peking Univ, Coll Engn, Dept Mat Sci & Engn, Beijing 100871, Peoples R China
3.Peking Univ, Acad Adv Interdisciplinary Studies, Coll Chem & Mol Engn, Ctr Nanochem CNC,Beijing Natl Lab Mol Sci, Beijing 100871, Peoples R China
4.Peking Univ, State Key Lab Artificial Microstruct & Mesoscop P, Beijing 100871, Peoples R China
5.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
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Zhou, Xiebo,Qi, Yue,Shi, Jianping,et al. Modulating the Electronic Properties of Monolayer Graphene Using a Periodic Quasi-One-Dimensional Potential Generated by Hex-Reconstructed Au(001)[J]. ACS NANO,2016,10(8):7550-7557.
APA Zhou, Xiebo.,Qi, Yue.,Shi, Jianping.,Niu, Jingjing.,Liu, Mengxi.,...&Zhang, Yanfeng.(2016).Modulating the Electronic Properties of Monolayer Graphene Using a Periodic Quasi-One-Dimensional Potential Generated by Hex-Reconstructed Au(001).ACS NANO,10(8),7550-7557.
MLA Zhou, Xiebo,et al."Modulating the Electronic Properties of Monolayer Graphene Using a Periodic Quasi-One-Dimensional Potential Generated by Hex-Reconstructed Au(001)".ACS NANO 10.8(2016):7550-7557.
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