High-order harmonic and attosecond pulse generations from Rydberg state driven by the spatially inhomogeneous field
Liu, Hang2; Li, Yi1; Feng, Liqiang1,2,3; Meng, Fanshun1; Castle, R. S.1,2
刊名MODERN PHYSICS LETTERS B
2017-02-10
卷号31期号:4
关键词High-order Harmonic Generation Rydberg State Attosecond X-ray Pulse Spatially Inhomogeneous Field
ISSN号0217-9849
DOI10.1142/S0217984917500294
文献子类Article
英文摘要High-order harmonic spectra and attosecond pulse generation from Rydberg atom (He+) driven by the spatially inhomogeneous field have been theoretically investigated. (i) Firstly, with an electron initially in a single excited Rydberg state (nth), the harmonic yield can be enhanced due to the decreased ionization potential, and a maximum enhancement can be obtained when the initial state is prepared as the third excited state (n = 3). However, the low cutoff energy from the excited state is unbeneficial to the generation of the higher photon pulse. Thus, with the further introduction of the laser chirp, not only the harmonic cutoff is extended, but also the harmonic modulation is reduced. As a result, five super-bandwidths from 63 eV to 267 eV can be found. (ii) Secondly, by preparing the initial state as a coherent superposition of excited state, the harmonic yield can be further enhanced, especially for the coherent superposition of the first and the third (n = 1 + 3) and the second and the fourth (n = 2 + 4) excited states, the harmonic yield is enhanced by 4-8 orders of magnitude compared with the case of the single ground initial state. Furthermore, by properly adding the laser pulse into the spatially inhomogeneous region (gap center x(0) = 0.0 a.u.) from left (x(0) < 0.0 a.u.) to right (x(0) > 0.0 a.u.), much higher cutoff energies can be obtained in the left region. As a consequence, two super-bandwidths of 248 eV and 496 eV can be obtained. Finally, by properly superposing the harmonics, a series of sub-25-as pulses with intensity enhancement of 5-8 orders of magnitude can be produced.
WOS关键词NONLINEAR OPTICS ; ENHANCEMENT ; ATOM
WOS研究方向Physics
语种英语
出版者WORLD SCIENTIFIC PUBL CO PTE LTD
WOS记录号WOS:000395126600008
内容类型期刊论文
源URL[http://cas-ir.dicp.ac.cn/handle/321008/169374]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Feng, Liqiang
作者单位1.Liaoning Univ Technol, Coll Sci, Jinzhou 121000, Liaoning, Peoples R China
2.Liaoning Univ Technol, Sch Chem & Environm Engn, Jinzhou 121000, Liaoning, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714
Liu, Hang,Li, Yi,Feng, Liqiang,et al. High-order harmonic and attosecond pulse generations from Rydberg state driven by the spatially inhomogeneous field[J]. MODERN PHYSICS LETTERS B,2017,31(4).
APA Liu, Hang,Li, Yi,Feng, Liqiang,Meng, Fanshun,&Castle, R. S..(2017).High-order harmonic and attosecond pulse generations from Rydberg state driven by the spatially inhomogeneous field.MODERN PHYSICS LETTERS B,31(4).
MLA Liu, Hang,et al."High-order harmonic and attosecond pulse generations from Rydberg state driven by the spatially inhomogeneous field".MODERN PHYSICS LETTERS B 31.4(2017).
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