Carbon dioxide reforming of methane over cobalt catalysts supported on hydrotalcite and metal oxides | |
Wang, Zhou-jun2; Bai, Xiaoli2; Guo, Yu2; Lu, Junying2; Gao, Lijun1; Liu, Qirui2; Tu, Weixia2 | |
刊名 | CATALYSIS COMMUNICATIONS
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2018-11-01 | |
卷号 | 116页码:81-84 |
关键词 | Cobalt Hydrotalcite MgO Al2O3 Dry reforming Syngas |
ISSN号 | 1566-7367 |
DOI | 10.1016/j.catcom.2018.08.017 |
通讯作者 | Wang, Zhou-jun(wangzj@mail.buct.edu.cn) |
英文摘要 | Cobalt (Co) catalysts supported on hydrotalcite (MgAl) and metal oxides (MgO, Al2O3) have been synthesized by co-precipitation methods for CO2 reforming of methane. It is found that the Co/MgAl catalyst possessed excellent initial activity and outstanding long-term stability. An activation process was observed on the Co/MgO catalyst, which was followed by moderate deactivation. The Co/Al2O3 catalyst suffered severe deactivation although it exhibited relatively good initial activity. The structural characterizations demonstrate that the exceptional reforming performance of the Co/MgAl catalyst was related to high specific surface area, abundant medium basic sites, tiny Co nanoparticles and strong metal-support interactions. |
资助项目 | National Natural Science Foundation of China[21811530293] ; National Natural Science Foundation of China[21776007] ; National Natural Science Foundation of China[21403012] |
WOS关键词 | HYDROGEN-PRODUCTION ; NI ; TEMPERATURE ; PERFORMANCE ; CO |
WOS研究方向 | Chemistry |
语种 | 英语 |
出版者 | ELSEVIER SCIENCE BV |
WOS记录号 | WOS:000444933100017 |
资助机构 | National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China |
内容类型 | 期刊论文 |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/167042] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
通讯作者 | Wang, Zhou-jun |
作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, iChEM, Dalian 116023, Peoples R China 2.Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing Key Lab Energy Environm Catalysis, Beijing 100029, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Zhou-jun,Bai, Xiaoli,Guo, Yu,et al. Carbon dioxide reforming of methane over cobalt catalysts supported on hydrotalcite and metal oxides[J]. CATALYSIS COMMUNICATIONS,2018,116:81-84. |
APA | Wang, Zhou-jun.,Bai, Xiaoli.,Guo, Yu.,Lu, Junying.,Gao, Lijun.,...&Tu, Weixia.(2018).Carbon dioxide reforming of methane over cobalt catalysts supported on hydrotalcite and metal oxides.CATALYSIS COMMUNICATIONS,116,81-84. |
MLA | Wang, Zhou-jun,et al."Carbon dioxide reforming of methane over cobalt catalysts supported on hydrotalcite and metal oxides".CATALYSIS COMMUNICATIONS 116(2018):81-84. |
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