Low threshold two-photon-pumped amplified spontaneous emission in ch3nh3pbbr3 microdisks | |
Yang, Bin1,2; Mao, Xin1,2; Yang, Songqiu1; Li, Yajuan1,2; Wang, Yanqiu1; Wang, Meishan3; Deng, Weiqiao1; Han, Keli1 | |
刊名 | Acs applied materials & interfaces |
2016-08-03 | |
卷号 | 8期号:30页码:19587-19592 |
关键词 | Amplified spontaneous emission Ch3nh3pbbr3 Perovskite Recombination Solution processed |
ISSN号 | 1944-8244 |
DOI | 10.1021/acsami.6b04246 |
通讯作者 | Han, keli(klhan@dicp.ac.cn) |
英文摘要 | Two-photon-pumped amplified spontaneous, emission (ase) of ch3nh3pbbr3 microdisks (mds) were investigated by using femtosecond laser system. low threshold at 2.2 mj cm(-2) was obtained. also, emission spectral tunability from 500 to 570 nm was demonstrated by synthesis the mixed halide perovskite mds. the spatial effect of photoluminescence (pl) properties under one photon and two-photon excitation were also studied by means of two-photon laser scanning microscope (tplsm) and time-resolved pl spectroscopy. it was found that the band to band emission of near-surface regions and photocarriers' diffusion from near-surface regions to interior regions is significant for one-photon excitation. by contrast, reabsorption of emission under two-photon excitation plays a major role in the emission properties of the mds. these results will give a more comprehensive understanding of the nonlinear effect of ch3nh3pbbr3 single crystals. |
WOS关键词 | PEROVSKITE SINGLE-CRYSTALS ; HALIDE PEROVSKITE ; STIMULATED-EMISSION ; QUANTUM DOTS ; COLLOIDAL NANOPLATELETS ; NONLINEAR ABSORPTION ; CARRIER DIFFUSION ; I CRYSTALS ; RECOMBINATION ; NANOCRYSTALS |
WOS研究方向 | Science & Technology - Other Topics ; Materials Science |
WOS类目 | Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
语种 | 英语 |
出版者 | AMER CHEMICAL SOC |
WOS记录号 | WOS:000380968300047 |
内容类型 | 期刊论文 |
URI标识 | http://www.corc.org.cn/handle/1471x/2375289 |
专题 | 中国科学院大学 |
通讯作者 | Han, Keli |
作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100039, Peoples R China 3.Ludong Univ, Sch Phys & Optoelect Engn, Yantai 264025, Peoples R China |
推荐引用方式 GB/T 7714 | Yang, Bin,Mao, Xin,Yang, Songqiu,et al. Low threshold two-photon-pumped amplified spontaneous emission in ch3nh3pbbr3 microdisks[J]. Acs applied materials & interfaces,2016,8(30):19587-19592. |
APA | Yang, Bin.,Mao, Xin.,Yang, Songqiu.,Li, Yajuan.,Wang, Yanqiu.,...&Han, Keli.(2016).Low threshold two-photon-pumped amplified spontaneous emission in ch3nh3pbbr3 microdisks.Acs applied materials & interfaces,8(30),19587-19592. |
MLA | Yang, Bin,et al."Low threshold two-photon-pumped amplified spontaneous emission in ch3nh3pbbr3 microdisks".Acs applied materials & interfaces 8.30(2016):19587-19592. |
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