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Low threshold two-photon-pumped amplified spontaneous emission in ch3nh3pbbr3 microdisks
Yang, Bin1,2; Mao, Xin1,2; Yang, Songqiu1; Li, Yajuan1,2; Wang, Yanqiu1; Wang, Meishan3; Deng, Weiqiao1; Han, Keli1
刊名Acs applied materials & interfaces
2016-08-03
卷号8期号:30页码:19587-19592
关键词Amplified spontaneous emission Ch3nh3pbbr3 Perovskite Recombination Solution processed
ISSN号1944-8244
DOI10.1021/acsami.6b04246
通讯作者Han, keli(klhan@dicp.ac.cn)
英文摘要Two-photon-pumped amplified spontaneous, emission (ase) of ch3nh3pbbr3 microdisks (mds) were investigated by using femtosecond laser system. low threshold at 2.2 mj cm(-2) was obtained. also, emission spectral tunability from 500 to 570 nm was demonstrated by synthesis the mixed halide perovskite mds. the spatial effect of photoluminescence (pl) properties under one photon and two-photon excitation were also studied by means of two-photon laser scanning microscope (tplsm) and time-resolved pl spectroscopy. it was found that the band to band emission of near-surface regions and photocarriers' diffusion from near-surface regions to interior regions is significant for one-photon excitation. by contrast, reabsorption of emission under two-photon excitation plays a major role in the emission properties of the mds. these results will give a more comprehensive understanding of the nonlinear effect of ch3nh3pbbr3 single crystals.
WOS关键词PEROVSKITE SINGLE-CRYSTALS ; HALIDE PEROVSKITE ; STIMULATED-EMISSION ; QUANTUM DOTS ; COLLOIDAL NANOPLATELETS ; NONLINEAR ABSORPTION ; CARRIER DIFFUSION ; I CRYSTALS ; RECOMBINATION ; NANOCRYSTALS
WOS研究方向Science & Technology - Other Topics ; Materials Science
WOS类目Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000380968300047
内容类型期刊论文
URI标识http://www.corc.org.cn/handle/1471x/2375289
专题中国科学院大学
通讯作者Han, Keli
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
3.Ludong Univ, Sch Phys & Optoelect Engn, Yantai 264025, Peoples R China
推荐引用方式
GB/T 7714
Yang, Bin,Mao, Xin,Yang, Songqiu,et al. Low threshold two-photon-pumped amplified spontaneous emission in ch3nh3pbbr3 microdisks[J]. Acs applied materials & interfaces,2016,8(30):19587-19592.
APA Yang, Bin.,Mao, Xin.,Yang, Songqiu.,Li, Yajuan.,Wang, Yanqiu.,...&Han, Keli.(2016).Low threshold two-photon-pumped amplified spontaneous emission in ch3nh3pbbr3 microdisks.Acs applied materials & interfaces,8(30),19587-19592.
MLA Yang, Bin,et al."Low threshold two-photon-pumped amplified spontaneous emission in ch3nh3pbbr3 microdisks".Acs applied materials & interfaces 8.30(2016):19587-19592.
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