A novel bioaccessibility prediction method for pahs in soil: composite extraction with hydroxypropyl-beta-cyclodextrin and extracellular polymer substances | |
Zhang, Yanan1,2; Yang, Xinglun1; Gu, Chenggang1; Wang, Fang1; Bian, Yongrong1; Song, Yang1; Wang, Daizhang3; Jiang, Xin1 | |
刊名 | Science of the total environment |
2016-11-01 | |
卷号 | 569页码:997-1003 |
关键词 | Bioaccessibility Composite extraction Hydroxypropyl-beta-cyclodextrin Rhamnolipid Bovine serum albumin Alginate sodium |
ISSN号 | 0048-9697 |
DOI | 10.1016/j.scitotenv.2016.05.226 |
通讯作者 | Jiang, xin(jiangxin@issas.ac.cn) |
英文摘要 | Hydroxypropyl-beta-cyclodextrin (hpcd) extraction has been widely used to estimate bioaccessibility of polycyclic aromatic hydrocarbons (pahs) in soil, but it often underestimates the actual risk due to lack of information regarding the exogenous active substances, such as extracellular polymer substance (eps) secreted by microorganisms. in this study, a novel technique, composite extraction of hpcd each with rhamnolipid (rl), bovine serum albumin (bsa) and alginate sodium(as), models of lipopolysaccharide, proteins and polysaccharides, was developed to assess pahs bioaccessibility to earthworms. in addition, comparisons were conducted with accelerated solvent extraction (ase) and individual hpcd extraction. the results demonstrated that all chemical extractions were linearly correlated with earthworm accumulation, and individual hpcd extraction underestimated pah bioaccessibility by about two times. however, the overall performances of the three composite chemical extractions (hpcd/as, hpcd/rl, hpcd/bsa) were better than individual hpcd extraction, among which, hpcd/as was best at estimating the earthworm accumulation (considering both correlation coefficient and fitted linear slope). therefore, all observations implied that hpcd/as extraction could be used as a fast and reliable method to predict pah bioaccessibility to earthworms in contaminated soils. (c) 2016 published by elsevier b.v. |
WOS关键词 | POLYCYCLIC AROMATIC-HYDROCARBONS ; POTENTIALLY TOXIC ELEMENTS ; SEWAGE-SLUDGE BIOCHAR ; HUMAN SERUM-ALBUMIN ; SODIUM ALGINATE ; AQUEOUS-SOLUTIONS ; CONTAMINATED SOILS ; PASSIVE SAMPLERS ; EISENIA-FOETIDA ; TRITON X-100 |
WOS研究方向 | Environmental Sciences & Ecology |
WOS类目 | Environmental Sciences |
语种 | 英语 |
出版者 | ELSEVIER SCIENCE BV |
WOS记录号 | WOS:000382269000096 |
内容类型 | 期刊论文 |
URI标识 | http://www.corc.org.cn/handle/1471x/2375243 |
专题 | 中国科学院大学 |
通讯作者 | Jiang, Xin |
作者单位 | 1.Chinese Acad Sci, Inst Soil Sci, Key Lab Soil Environm & Pollut Remediat, Nanjing 210008, Jiangsu, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Henan Agr Univ, Coll Resources & Environm, Zhengzhou 450002, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Yanan,Yang, Xinglun,Gu, Chenggang,et al. A novel bioaccessibility prediction method for pahs in soil: composite extraction with hydroxypropyl-beta-cyclodextrin and extracellular polymer substances[J]. Science of the total environment,2016,569:997-1003. |
APA | Zhang, Yanan.,Yang, Xinglun.,Gu, Chenggang.,Wang, Fang.,Bian, Yongrong.,...&Jiang, Xin.(2016).A novel bioaccessibility prediction method for pahs in soil: composite extraction with hydroxypropyl-beta-cyclodextrin and extracellular polymer substances.Science of the total environment,569,997-1003. |
MLA | Zhang, Yanan,et al."A novel bioaccessibility prediction method for pahs in soil: composite extraction with hydroxypropyl-beta-cyclodextrin and extracellular polymer substances".Science of the total environment 569(2016):997-1003. |
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