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Aqueous based semiconductor nanocrystals
Jing, Lihong1; Kershaw, Stephen V.2,3; Li, Yilin4; Huang, Xiaodan1,5; Li, Yingying1,5; Rogach, Andrey L.2,3; Gao, Mingyuan1,5
刊名Chemical reviews
2016-09-28
卷号116期号:18页码:10623-10730
ISSN号0009-2665
DOI10.1021/acs.chemrev.6b00041
通讯作者Rogach, andrey l.(andrey.rogach@cityu.edu.hk) ; Gao, mingyuan(gaomy@iccas.ac.cn)
英文摘要This review summarizes traditional and recent nonconventional, bioinspired, methods for the aqueous synthesis of colloidal semiconductor quantum dots (qds). the basic chemistry concepts are critically emphasized at the very beginning as these are strongly correlated with the selection of ligands and the optimal formation of aqueous qds and their more sophisticated structures. the synergies of biomimetic and biosynthetic methods that can combine biospecific reactivity with the robust and strong optical responses of qds have also resulted in new approaches to the synthesis of the nanoparticles themselves. a related new avenue is the recent extension of qd synthesis to form nanoparticles endowed with chiral optical properties. the optical characteristics of qd materials and their advanced forms such as core/shell heterostructures, alloys, and doped qds are discussed: from the design considerations of optical band gap tuning, the control and reduction of the impact of surface traps, the consideration of charge carrier processes that affect emission and energy and charge transfer, to the impact and influence of lattice strain. we also describe the considerable progress in some selected qd applications such as in bioimaging and theranostics. the review concludes with future strategies and identification of key challenges that still need to be resolved in reaching very attractive, scalable, yet versatile aqueous syntheses that may widen the scope of commercial applications for semiconductor nanocrystals.
WOS关键词CORE/SHELL QUANTUM DOTS ; CORE-SHELL NANOCRYSTALS ; MICROWAVE-ASSISTED SYNTHESIS ; ONE-POT SYNTHESIS ; NEAR-INFRARED FLUORESCENCE ; CAPPED CDTE NANOCRYSTALS ; MN-DOPED ZNSE ; CADMIUM-SULFIDE NANOPARTICLES ; SENSITIZED SOLAR-CELLS ; LIGHT-EMITTING-DIODES
WOS研究方向Chemistry
WOS类目Chemistry, Multidisciplinary
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000384518600006
内容类型期刊论文
URI标识http://www.corc.org.cn/handle/1471x/2375031
专题中国科学院大学
通讯作者Rogach, Andrey L.; Gao, Mingyuan
作者单位1.Chinese Acad Sci, Inst Chem, Bei Yi Jie 2, Beijing 100190, Peoples R China
2.City Univ Hong Kong, Dept Phys & Mat Sci, 83 Tat Chee Ave, Kowloon, Hong Kong, Peoples R China
3.City Univ Hong Kong, Ctr Funct Photon, 83 Tat Chee Ave, Kowloon, Hong Kong, Peoples R China
4.Peking Univ, Canc Hosp & Inst, Dept GI Oncol, Key Lab Carcinogenesis & Translat Res, Fucheng Rd 52, Beijing 100142, Peoples R China
5.Univ Chinese Acad Sci, Sch Chem & Chem Engn, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Jing, Lihong,Kershaw, Stephen V.,Li, Yilin,et al. Aqueous based semiconductor nanocrystals[J]. Chemical reviews,2016,116(18):10623-10730.
APA Jing, Lihong.,Kershaw, Stephen V..,Li, Yilin.,Huang, Xiaodan.,Li, Yingying.,...&Gao, Mingyuan.(2016).Aqueous based semiconductor nanocrystals.Chemical reviews,116(18),10623-10730.
MLA Jing, Lihong,et al."Aqueous based semiconductor nanocrystals".Chemical reviews 116.18(2016):10623-10730.
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