Dynamical interference in the vibronic bond breaking reaction of hco | |
Han, Shanyu1,2; Zheng, Xianfeng3,4; Ndengue, Steve5; Song, Yu4; Dawes, Richard5; Xie, Daiqian1,6,7,8; Zhang, Jingsong4; Guo, Hua2 | |
刊名 | Science advances |
2019 | |
卷号 | 5期号:1页码:6 |
ISSN号 | 2375-2548 |
DOI | 10.1126/sciadv.aau0582 |
通讯作者 | Dawes, richard(dawesr@mst.edu) ; Xie, daiqian(dqxie@nju.edu.cn) ; Zhang, jingsong(jingsong.zhang@ucr.edu) ; Guo, hua(hguo@unm.edu) |
英文摘要 | First-principles treatments of quantum molecular reaction dynamics have reached the level of quantitative accuracy even in cases with strong non-born-oppenheimer effects. this achievement permits the interpretation of puzzling experimental phenomena related to dynamics governed by multiple coupled potential energy surfaces. we present a combined experimental and theoretical study of the photodissociation of formyl radical (hco). oscillations observed in the distribution of product states are found to arise from the interference of matter waves-a manifestation analogous to young's double-slit experiment. |
WOS关键词 | STATE PHOTODISSOCIATION DYNAMICS ; POTENTIAL-ENERGY SURFACE ; 1ST ABSORPTION-BAND ; RENNER-TELLER ; AB-INITIO ; UNIMOLECULAR DISSOCIATION ; TRIATOMIC-MOLECULES ; DISTRIBUTIONS ; SPECTROSCOPY ; TRANSITION |
WOS研究方向 | Science & Technology - Other Topics |
WOS类目 | Multidisciplinary Sciences |
语种 | 英语 |
出版者 | AMER ASSOC ADVANCEMENT SCIENCE |
WOS记录号 | WOS:000457547900003 |
内容类型 | 期刊论文 |
URI标识 | http://www.corc.org.cn/handle/1471x/2372806 |
专题 | 大连化学物理研究所 |
通讯作者 | Dawes, Richard; Xie, Daiqian; Zhang, Jingsong; Guo, Hua |
作者单位 | 1.Nanjing Univ, Sch Chem & Chem Engn, Key Lab Mesoscop Chem, Inst Theoret & Computat Chem, Nanjing 210093, Jiangsu, Peoples R China 2.Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA 3.Anhui Normal Univ, Dept Phys, Anhui Prov Key Lab Optoelect Mat Sci & Technol, Wuhu 241000, Anhui, Peoples R China 4.Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA 5.Missouri Univ Sci & Technol, Dept Chem, Rolla, MO 65409 USA 6.Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China 7.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China 8.Chinese Acad Sci, Dalian Inst Chem Phys, Ctr Theoret Computat Chem, Dalian 116023, Peoples R China |
推荐引用方式 GB/T 7714 | Han, Shanyu,Zheng, Xianfeng,Ndengue, Steve,et al. Dynamical interference in the vibronic bond breaking reaction of hco[J]. Science advances,2019,5(1):6. |
APA | Han, Shanyu.,Zheng, Xianfeng.,Ndengue, Steve.,Song, Yu.,Dawes, Richard.,...&Guo, Hua.(2019).Dynamical interference in the vibronic bond breaking reaction of hco.Science advances,5(1),6. |
MLA | Han, Shanyu,et al."Dynamical interference in the vibronic bond breaking reaction of hco".Science advances 5.1(2019):6. |
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