Atmospheric occurrence and health risks of PCDD/Fs, polychlorinated biphenyls, and polychlorinated naphthalenes by air inhalation in metallurgical plants | |
Yang, Lili; Liu, Guorui; Zheng, Minghui; Jin, Rong; Zhu, Qingqing; Zhao, Yuyang; Zhang, Xian; Xu, Yang | |
刊名 | SCIENCE OF THE TOTAL ENVIRONMENT |
2017-03-01 | |
卷号 | 580期号:0页码:1146-1154 |
关键词 | Persistent Organic Pollutants Polychlorinated Dibenzo-p-dioxins And Dibenzofurans (Pcdd/fs) Polychlorinated Biphenyls (Pcbs) Polychlorinated Naphthalenes (Pcns) Metallurgical Sources Inhalation Risk |
英文摘要 | Metallurgical plants are important sources of polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs), polychlorinated biphenyls (PCBs) and polychlorinated naphthalenes (PCNs). It is significant to evaluate the air levels and human risks of PCDD/Fs, PCBs and PCNs in metallurgical plants considering their adverse effects on human health and thousands of metallurgical plants being in operation in China. The estimated inhalation intakes of PCDD/Fs, PCBs, and PCNs together in eight iron ore sintering plants, three secondary copper plants, four secondary aluminum plants, and one secondary lead plant were 4.9-213.4, 21.4-4026.4, 28.7-630, and 11.7 fg TEQ kg(-1) day(-1), respectively, and the corresponding cancer risks were estimated to be 8.7 x 10(-7) to 3.8 x 10(-5), 5.1 x 10(-6) to 1.1 x 10(-4), 3.8 x 10(-6) to 7.1 x 10(-4), and 2.1 x 10(-6), respectively. The estimated cancer risk were higher than 100 per million people for three secondary aluminum and copper smelters among the sixteen metallurgical plants, indicating high cancer risks. Stack gas samples from metallurgical plants were also collected and analyzed for comparing their emission profiles with that of air samples. The comparison of PCDD/F, PCB and PCN profiles between air samples and stack gas samples by similarity calculation and principal component analysis suggested the influence of stack gas emissions from metallurgical plants on surrounding air. These results are helpful for understanding the exposure risk to PCDD/Fs, PCBs and PCNs in numerous metallurgical plants being operation in China. (C) 2016 Elsevier B.V. All rights reserved. |
内容类型 | 期刊论文 |
源URL | [http://ir.rcees.ac.cn/handle/311016/39253] |
专题 | 生态环境研究中心_环境化学与生态毒理学国家重点实验室 |
推荐引用方式 GB/T 7714 | Yang, Lili,Liu, Guorui,Zheng, Minghui,et al. Atmospheric occurrence and health risks of PCDD/Fs, polychlorinated biphenyls, and polychlorinated naphthalenes by air inhalation in metallurgical plants[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2017,580(0):1146-1154. |
APA | Yang, Lili.,Liu, Guorui.,Zheng, Minghui.,Jin, Rong.,Zhu, Qingqing.,...&Xu, Yang.(2017).Atmospheric occurrence and health risks of PCDD/Fs, polychlorinated biphenyls, and polychlorinated naphthalenes by air inhalation in metallurgical plants.SCIENCE OF THE TOTAL ENVIRONMENT,580(0),1146-1154. |
MLA | Yang, Lili,et al."Atmospheric occurrence and health risks of PCDD/Fs, polychlorinated biphenyls, and polychlorinated naphthalenes by air inhalation in metallurgical plants".SCIENCE OF THE TOTAL ENVIRONMENT 580.0(2017):1146-1154. |
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