Relativistic coupled-cluster calculations of the polarizabilities of atomic thallium

doi:10.1103/PhysRevA.98.062511

	Relativistic coupled-cluster calculations of the polarizabilities of atomic thallium
	Shi, Ting-Yun 1; Lou, Bing-Qiong 2; Gao, Ning-Ning 2; Tang, Yong-Bo 1,2
刊名	PHYSICAL REVIEW A
	2018-12-14
卷号	98 期号:6 页码:9
ISSN号	2469-9926
DOI	10.1103/PhysRevA.98.062511
英文摘要	Using the relativistic coupled-cluster method, we calculate the static dipole polarizabilities of the 6p, 7s, 7p, 8s, 8p, and 6d states and the dynamic dipole polarizabilities of the 6p and 7s states of the thallium atom. The trivalent thallium atom is computationally treated as a monovalent system, together with all linear and nonlinear terms of single- and double-cluster operators included in the correlation calculations. We observe that the dominating contributions to the static scalar polarizabilities of the 7s(1/2), 7p(1/2), 8p(1/2), and 8p(3/2) states are from one or two specific transitions. The matrix elements of these specific transitions can be determined by combining the experimental values of relevant static scalar polarizabilities. A number of magic wavelengths for the 6p(1/2)-7s and 6p(3/2)-7s transitions in the range of 488-1300 nm and the longest tune-out wavelength of the ground state are determined. These magic wavelengths and tune-out wavelength may be useful for further thallium experiments. Experimental measurements of the magic wavelengths near 1245 nm would give estimates of the 7s(1/2)-7p(1/2) and 7s(1/2)-7p(3/2) transition matrix elements and their ratio. Furthermore, lifetimes of many excited states, as well as the Stark-induced scalar and vector dipole polarizabilities for the 6p(1/2)-7p(1/2) transition, are also evaluated and compared with available theoretical and experimental values.
资助项目	National Natural Science Foundation of China[11504094] ; National Natural Science Foundation of China[91536102] ; Chinese Academy of Sciences[XDB21030300] ; China Postdoctoral Science Foundation[2017M622556]
WOS关键词	LIFETIMES ; TRANSITION
WOS研究方向	Optics ; Physics
语种	英语
出版者	AMER PHYSICAL SOC
WOS记录号	WOS:000453456400004
资助机构	National Natural Science Foundation of China ; National Natural Science Foundation of China ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation
内容类型	期刊论文
源URL	[http://ir.wipm.ac.cn/handle/112942/13500]
专题	中国科学院武汉物理与数学研究所
通讯作者	Tang, Yong-Bo
作者单位	1.Chinese Acad Sci, Wuhan Inst Phys & Math, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Hubei, Peoples R China 2.Henan Normal Univ, Coll Phys & Elect Engn, Xinxiang 453007, Peoples R China
推荐引用方式 GB/T 7714	Shi, Ting-Yun,Lou, Bing-Qiong,Gao, Ning-Ning,et al. Relativistic coupled-cluster calculations of the polarizabilities of atomic thallium[J]. PHYSICAL REVIEW A,2018,98(6):9.
APA	Shi, Ting-Yun,Lou, Bing-Qiong,Gao, Ning-Ning,&Tang, Yong-Bo.(2018).Relativistic coupled-cluster calculations of the polarizabilities of atomic thallium.PHYSICAL REVIEW A,98(6),9.
MLA	Shi, Ting-Yun,et al."Relativistic coupled-cluster calculations of the polarizabilities of atomic thallium".PHYSICAL REVIEW A 98.6(2018):9.