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	Yin-Yang Harmony: Metal and Nonmetal Dual-Doping Boosts Electrocatalytic Activity for Alkaline Hydrogen Evolution
	Xu, Kun1; Sun, Yiqiang2; Sun, Yuanmiao3; Zhang, Yongqi1; Jia, Guichong1; Zhang, Qinghua4; Gu, Lin4; Li, Shuzhou3; Li, Yue2; Fan, Hong Jin1
刊名	ACS ENERGY LETTERS
	2018-11-01
卷号	3期号:11页码:2750-2756
ISSN号	2380-8195
DOI	10.1021/acsenergylett.8b01893
通讯作者	Li, Yue(yueli@issp.ac.cn) ; Fan, Hong Jin(fanhj@ntu.edu.sg)
英文摘要	Active site number, water dissociation, and hydrogen adsorption free energy are the three main parameters for regulating the activity of electrocatalysts for hydrogen evolution reaction (HER) in alkaline media. However, at present, simultaneous modulations of these three parameters for alkaline HER still remain challenging. In this work, we take CoP as the model material and demonstrate that a metal and nonmetal dual-doping strategy can achieve simultaneous modulation of these three parameters by inducing lattice irregularity and optimizing the electronic configuration in CoP nanomaterials. Benefiting from the oxygen and copper dual-doping collective effect, the optimized O,Cu-CoP nanowire array electrode shows nearly 10-fold enhancement in catalytic activity for alkaline HER compared to a pure CoP nanowire electrode. Our work may provide a new concept to boost performance of nonprecious metal electrocatalysts for alkaline HER.
资助项目	Singapore MOE AcRF Tier 2 Grant[MOE2017-T2-1-073] ; National Natural Science Foundation of China[51728204]
WOS关键词	ENHANCED CATALYTIC-ACTIVITY ; OXYGEN EVOLUTION ; EFFICIENT ; CHALLENGES ; NANOSHEETS ; COPPER ; COSE2
WOS研究方向	Chemistry ; Electrochemistry ; Energy & Fuels ; Science & Technology - Other Topics ; Materials Science
语种	英语
出版者	AMER CHEMICAL SOC
WOS记录号	WOS:000450374600017
资助机构	Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; Singapore MOE AcRF Tier 2 Grant ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China
内容类型	期刊论文
源URL	[http://ir.hfcas.ac.cn:8080/handle/334002/34402]
专题	合肥物质科学研究院_中科院固体物理研究所
通讯作者	Li, Yue; Fan, Hong Jin
作者单位	1.Nanyang Technol Univ, Sch Phys & Math Sci, 21 Nanyang Link, Singapore 637371, Singapore 2.Chinese Acad Sci, Inst Solid State Phys, Anhui Key Lab Nanomat & Nanotechnol, Key Lab Mat Phys, Hefei 230031, Anhui, Peoples R China 3.Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore 4.Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China
推荐引用方式 GB/T 7714	Xu, Kun,Sun, Yiqiang,Sun, Yuanmiao,et al. Yin-Yang Harmony: Metal and Nonmetal Dual-Doping Boosts Electrocatalytic Activity for Alkaline Hydrogen Evolution[J]. ACS ENERGY LETTERS,2018,3(11):2750-2756.
APA	Xu, Kun.,Sun, Yiqiang.,Sun, Yuanmiao.,Zhang, Yongqi.,Jia, Guichong.,...&Fan, Hong Jin.(2018).Yin-Yang Harmony: Metal and Nonmetal Dual-Doping Boosts Electrocatalytic Activity for Alkaline Hydrogen Evolution.ACS ENERGY LETTERS,3(11),2750-2756.
MLA	Xu, Kun,et al."Yin-Yang Harmony: Metal and Nonmetal Dual-Doping Boosts Electrocatalytic Activity for Alkaline Hydrogen Evolution".ACS ENERGY LETTERS 3.11(2018):2750-2756.

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