Heavy-ion irradiation effects on Gd2Zr2O7 ceramics bearing complex nuclear waste

doi:10.1016/j.jallcom.2018.09.006

CORC > 合肥物质科学研究院 > 中国科学院合肥物质科学研究院 > 中科院等离子体物理研究所

	Heavy-ion irradiation effects on Gd2Zr2O7 ceramics bearing complex nuclear waste
	Lu, Xirui 1,2; Shu, Xiaoyan 1,2; Wang, Lan 2; Shao, Dadong 3; Zhang, Haibin 4; Zhang, Kuibao 1; Xie, Yi 3
刊名	JOURNAL OF ALLOYS AND COMPOUNDS
	2019-01-15
卷号	771 页码:973-979
关键词	Pyrochlore Gd2Zr2O7 TRPO waste Irradiation effects Phase transformation
ISSN号	0925-8388
DOI	10.1016/j.jallcom.2018.09.006
通讯作者	Lu, Xirui(luxirui@swust.edu.cn) ; Zhang, Haibin(wsschbinzhang@163.com)
英文摘要	The irradiation response of Gd2Zr2O7 ceramic bearing complex nuclear waste was explored by heavy ions to relatively high fluences. The Gd2Zr2O7 ceramic holding 25 wt.% and 40 wt.% of simulated TRPO waste (containing 11 kinds of oxides) were irradiated by 1.5 MeV Xe20+ to fluences ranging from 1.0 x 10(12) ions/cm(2) to 1.0 x 10(15) ions/cm(2) at room temperature. Irradiation induced structure disordering (i.e. phase transformation from pyrochlore to defect-fluorite and finally to amorphous structure) was disclosed by GIXRD, Raman and TEM. The results indicated the structure disordering was influenced by fluences, irradiation depth and waste loading content. This work identified the Gd2Zr2O7 ceramics as a potential candidate in immobilizing complex oxides from the aspect of irradiation tolerance. (c) 2018 Elsevier B.V. All rights reserved.
资助项目	National Natural Science Foundation of China, China[21507105] ; Key Project of Sichuan Education Department, China[15ZB0116] ; Longshan academic talent research supporting program of SWUST, China[18LZX312] ; Longshan academic talent research supporting program of SWUST, China[18LZX520]
WOS关键词	PYROCHLORE ; EXTRACTION ; AMORPHIZATION ; RADIONUCLIDES ; A(2)B(2)O(7) ; TRANSITION ; ACTINIDES ; PRESSURE ; DISORDER ; GD2TI2O7
WOS研究方向	Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering
语种	英语
出版者	ELSEVIER SCIENCE SA
WOS记录号	WOS:000449621500120
资助机构	National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; National Natural Science Foundation of China, China ; 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内容类型	期刊论文
源URL	[http://ir.hfcas.ac.cn:8080/handle/334002/34307]
专题	合肥物质科学研究院_中科院等离子体物理研究所
通讯作者	Lu, Xirui; Zhang, Haibin
作者单位	1.Southwest Univ Sci & Technol, State Key Lab Environm Friendly Energy Mat, Mianyang 621010, Sichuan, Peoples R China 2.Southwest Univ Sci & Technol, Fundamental Sci Nucl Wastes & Environm Safety Lab, Mianyang 621010, Peoples R China 3.Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Anhui, Peoples R China 4.China Acad Engn Phys, Inst Nucl Phys & Chem, Mianyang 621900, Peoples R China
推荐引用方式 GB/T 7714	Lu, Xirui,Shu, Xiaoyan,Wang, Lan,et al. Heavy-ion irradiation effects on Gd2Zr2O7 ceramics bearing complex nuclear waste[J]. JOURNAL OF ALLOYS AND COMPOUNDS,2019,771:973-979.
APA	Lu, Xirui.,Shu, Xiaoyan.,Wang, Lan.,Shao, Dadong.,Zhang, Haibin.,...&Xie, Yi.(2019).Heavy-ion irradiation effects on Gd2Zr2O7 ceramics bearing complex nuclear waste.JOURNAL OF ALLOYS AND COMPOUNDS,771,973-979.
MLA	Lu, Xirui,et al."Heavy-ion irradiation effects on Gd2Zr2O7 ceramics bearing complex nuclear waste".JOURNAL OF ALLOYS AND COMPOUNDS 771(2019):973-979.